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Lateral ion migration accelerates degradation in halide perovskite devices

Publications associées (45)

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Recent years have witnessed considerable progress in the development of solar cells based on lead halide perovskite materials. However, their intrinsic instability remains a limitation. In this context, the interplay between the thermal degradation and the ...

2019

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Since reaching 20% efficiency, research in perovskite photovoltaics has shifted from a race for efficiency to a race for stability. For efficiency, the standard test conditions set the rules for the race. However, the term 'stability' is used very broadly ...

NATURE PUBLISHING GROUP2019

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The stability of perovskite solar cells is a key issue for industrial development. One reason for this is the volatile organic methylammonium (MA) cation, which is prone to degas under elevated temperatures from the perovskite. At the same time, small amou ...

2019

Phosphonic Acid Modification of the Electron Selective Contact: Interfacial Effects in Perovskite Solar Cells

Wolfgang Richard Tress, Ulf Anders Hagfeldt, Juan-Pablo Correa-Baena, Silver Hamill Turren Cruz, Rebecca Hill

The role electron-transport layers (ETLs) play in perovskite solar cells (PSCs) is still widely debated. Conduction band alignment at the perovskite/ETL interface has been suggested to be an important role for the performance of the solar cells. However, l ...

AMER CHEMICAL SOC2019

High performance of both photovoltaic and electroluminescent devices requires low nonradiative recombination losses. In perovskites, such loses strongly depend on the carrier traps related to the mobile ions and vacancies, causing I-V hysteresis of solar c ...

AMER CHEMICAL SOC2019

Organic-inorganic lead halide perovskites have shown impressive power conversion efficiency (PCE) in a range of solar cell architectures. Despite the multiple ionic compositions that have been reported so far, the presence of organic constituents is an ess ...

2019

Perovskite solar cells (PSCs) have attracted a substantial interest owing to a very fast achievement of efficiencies >20 % within only several years of development. However, for any solar cell to become technologically viable, two additional milestones hav ...

EPFL2018

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In this study, we discuss the underlying mechanism of the current-voltage hysteresis in a hybrid lead-halide perovskite solar cell. We have developed a method based on Kelvin probe force microscopy that enables mapping charge redistribution in an operating ...

ROYAL SOC CHEMISTRY2018

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The surge of the power conversion efficiency of metal halide lead perovskite solar cells comes with concerns, such as the long-term ecotoxicity of lead compounds, their sensitivity toward moisture and oxygen, or the scarcity of some of their components. Mo ...

Wiley-Blackwell2017

Undoubtedly, perovskite solar cells have become a key player in 3rd generation photovoltaics over the last few years. Although it is only in 2012 that the first solid state perovskite solar cell was reported, power conversion efficiencies have increased so ...

EPFL2017

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