Quadrupolar susceptibility modeling of substrated metasurfaces with application to the generalized Brewster effect

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Wafer‐Scale Functional Metasurfaces for Mid‐Infrared Photonics and Biosensing

Hatice Altug, Aurélian Michel John-Herpin, Aleksandrs Leitis, Ming-Lun Tseng

Metasurfaces have emerged as a breakthrough platform for manipulating light at the nanoscale and enabling on-demand optical functionalities for next-generation biosensing, imaging, and light-generating photonic devices. However, translating this technology ...

Wiley2021

Structural and analytical identifications of biomolecules by cold ion spectroscopy of non-covalent complexes

Erik Saparbayev

Non-covalent interactions are ubiquitous in nature. The diversity and functionality of these interactions are employed by nature as a universal tool for building the molecular mechanism of life. Although weak, these interactions play a key role in both for ...

EPFL2021

DORI Reveals the Influence of Noncovalent Interactions on Covalent Bonding Patterns in Molecular Crystals Under Pressure

Berend Smit, Anne-Clémence Corminboeuf, Benjamin André René Meyer, Senja Dominique Barthel, Laurent Alexis Clément Vannay, Amber Kashan Mace

The study of organic molecular crystals under high pressure provides fundamental insight into crystal packing distortions and reveals mechanisms of phase transitions and the crystallization of polymorphs. These solid-state transformations can be monitored ...

2019

Interplay of H-Bonds with Aromatics in Isolated Complexes Identifies Isomeric Carbohydrates

Oleg Boyarkine, Ruslan Yamaletdinov, Vladimir Kopysov, Aleksandr Pereverzev

The tremendous isomeric diversity of carbohydrates enables a wide range of their biological functions but makes the identification and study of these molecules difficult. We investigated the ability of intermolecular interactions to communicate structural ...

Wiley-VCH Verlag GmbH2019

Accurate molecular polarizabilities with coupled cluster theory and machine learning

Michele Ceriotti, David Mark Wilkins, Andrea Grisafi, Yang Yang

The molecular dipole polarizability describes the tendency of a molecule to change its dipole moment in response to an applied electric field. This quantity governs key intra- and intermolecular interactions, such as induction and dispersion; plays a vital ...

2019

Extending the Scope of the Density Overlap Region Indicator

Laurent Alexis Clément Vannay

In this thesis, original applications of the Density Overlap Region Indicator (DORI), a density dependent bonding descriptor capable of simultaneously capturing covalent and noncovalent interactions, are discussed. The use of scalar fields, such as DORI, w ...

EPFL2018

Advanced Plasmonic Nanostructures for Engineering Fluorescence Applications

Xiaolong Wang

The appeal of plasmonics lies in the unique properties of coinage metal nanoparticles to strongly confine and enhance electromagnetic fields at the subwavelength. A simple 50 nm colloidal plasmonic particle can not only break the classical diffraction limi ...

EPFL2017

Multifunctional Plasmonic Metasurfaces for Novel Spectral and Spatial Applications

Chen Yan

Intensive developments of plasmonic nanomaterials over recent decades have inspired appealing applications in biosensing, optical trapping, fluorescence enhancement and light harvesting in solar cells. These nanostructures supporting unique light-matter in ...

EPFL2017

Subwavelength Focusing of Bloch Surface Waves

Hans Peter Herzig, Myun Sik Kim, Nicolas Maxime André Descharmes, Babak Vosoughi Lahijani

Microsized spheres can focus light into subwavelength spatial domains, a phenomenon called photonic nanojet. Even though well studied in three-dimensional (3D) configurations, only a few attempts have been reported to observe similar phenomena in two-dimen ...

Amer Chemical Soc2017

Origin of the Strong Interaction between Polar Molecules and Copper(II) Paddle-Wheels in Metal Organic Frameworks

Berend Smit, Daniele Ongari, Davide Tiana

The copper paddle-wheel is the building unit of many metal organic frameworks. Because of the ability of the copper cations to attract polar molecules, copper paddle-wheels are promising for carbon dioxide adsorption and separation. They have therefore bee ...

American Chemical Society2017

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