On the interaction of femtosecond laser pulses with layered dielectric materials
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The efficiency of classical gas-dynamic isotope sepn. can be strongly improved with the aid of a relatively weak IR laser. Irradn. in the collisional region of a free jet of SF6 dild. in Ar with a 20-W CO2 laser leads to an increase in the overall enrichme ...
SF6 in a free jet was vibrationally excited by a continuous-wave CO2 laser. The subsequent energy transfer processes, in which vibrational energy is degraded, lead to changes in the beam's spatial, velocity and cluster-size distributions. These changes wer ...
Unimol. reactions induced by absorption of multiple quanta of monochromatic IR radiation were studied on a model system comprising dissocn. of CF2HCl giving CF2 and HCl. Three expts. providing detailed information of IR multiphoton chem. were performed whi ...
The deposition of Ga on quartz substrates by photodissociation of trimethylgallium has been investigated. Light from a frequency doubled Ar-ion laser beam (257.2 nm) was focused onto quartz substrates. The Ar-ion laser was operated under CW or mode-locking ...
A simple energy-grained master equation was used to model data on the multiphoton dissocn. of CF2HCl as a function of laser fluence and Ar bath-gas pressure. Information on energy transfer from vibrationally excited CF2HCl was obtained from an anal. of the ...
A mol. beam mass spectrometer was constructed to study the formation of van der Waals clusters over a wide mass range. Using this app. (SF6)m was detected with 1 ? m ? 100 in the adiabatic expansion of SF6. By irradiating the SF6 jet with a continuous-wave ...
The IR multiphonon dissocn. of CF2HCl was investigated by monitoring the appearance of the CF2 product in real time during and after the laser pulse. The difluorcarbene radicals were detected quant. by their optical absorption in the ~A1B1->~X1A1 band syst ...
The output of an ideally mode-locked laser, namely, one having equal phase angles of the modes, consists of a train of bandwidth-limited short pulses. The influence of deviations from equal phase angles on the laser output is investigated. Random distribut ...
