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Alleviating nanostructural phase impurities enhances the optoelectronic properties, device performance and stability of cesium-formamidinium metal-halide perovskites

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Recent years have witnessed considerable progress in the development of solar cells based on lead halide perovskite materials. However, their intrinsic instability remains a limitation. In this context, the interplay between the thermal degradation and the ...

2019

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The role electron-transport layers (ETLs) play in perovskite solar cells (PSCs) is still widely debated. Conduction band alignment at the perovskite/ETL interface has been suggested to be an important role for the performance of the solar cells. However, l ...

AMER CHEMICAL SOC2019

Optoelectronic Properties of Layered Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Sanghyun Paek, Yonghui Lee, Kyung Taek Cho

Herein, the optoelectronic properties of interface-engineered perovskite 2D|3D-heterojunction structure solar cells are reported. The reciprocity theorem is applied to determine the maximum open-circuit voltage (V-oc) the device can deliver under solar ill ...

2019

Gate-tunable Scanning Tunneling Microscope as a tool for performing single-molecule chemistry

Shai Mangel

The atomic level understanding and control of the electron transport has important advantages for many applications, such as molecular electronics, solar cells and sensors. The target of my Ph.D. work is to investigate electronic and chemical properties of ...

EPFL2019

Performance of perovskite solar cells under simulated temperature-illumination real-world operating conditions

Michael Graetzel, Wolfgang Richard Tress, Ulf Anders Hagfeldt, Konrad Domanski, Essa Awadh R Alharbi, Brian Irving Carlsen, Anand Agarwalla

Since reaching 20% efficiency, research in perovskite photovoltaics has shifted from a race for efficiency to a race for stability. For efficiency, the standard test conditions set the rules for the race. However, the term 'stability' is used very broadly ...

NATURE PUBLISHING GROUP2019

A chain is as strong as its weakest link - Stability study of MAPbI(3) under light and temperature

Michael Graetzel, Ulf Anders Hagfeldt, Michael Saliba, Pankaj Kumar Yadav, Amita Ummadisingu, Silver Hamill Turren Cruz, Philippe Jürgen Holzhey

The stability of perovskite solar cells is a key issue for industrial development. One reason for this is the volatile organic methylammonium (MA) cation, which is prone to degas under elevated temperatures from the perovskite. At the same time, small amou ...

2019

Today more than 90% of the global PV market is covered by c-Si solar cells which are limited by recombination losses at the metal-semiconductor interface. This recombination path can be avoided by separating the metal from the c-Si wafer by introducing a b ...

EPFL2018

Hill climbing hysteresis of perovskite-based solar cells: a maximum power point tracking investigation

Michael Graetzel, Shaik Mohammed Zakeeruddin, Fabrizio Giordano, Joachim Maier, Mohammad Ibrahim Dar, Norman Pellet

The surge of the power conversion efficiency of metal halide lead perovskite solar cells comes with concerns, such as the long-term ecotoxicity of lead compounds, their sensitivity toward moisture and oxygen, or the scarcity of some of their components. Mo ...

Wiley-Blackwell2017

Inorganic-organic lead-halide perovskite solar cells have reached efficiencies above 22% within a few years of research. Achieved photovoltages of >1.2 V are outstanding for a material with a bandgap of 1.6 eV - in particular considering that it is solutio ...

Wiley-V C H Verlag Gmbh2017

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Hydrogenated amorphous silicon (alpha-Si:H) has been used for decades doped and as intrinsic absorber layers in thin-film silicon solar cells. Whereas their effiency was improved for a long time by the deposition of higher quality absorber layers, recent i ...

Elsevier2017