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Carbon nano-onions are a class of nanomaterials that can exhibit long electron spin relaxation times at room temperature and thus hold promise as potential building blocks for spintronics and quantum information processing devices. Despite first being synt ...
We photoexcite high-energy holon-doublon pairs as a way to alter the magnetic free energy landscape and resulting phase diagram of the frustrated honeycomb magnet ??-RuCl3. The pair recombination through multimagnon emission is tracked through the time evo ...
The dynamics of the S = 3/2 kagome antiferromagnet chromium jarosite, KCr3(OD)(6)(SO4)(2), was studied using high-resolution neutron time-of-flight spectroscopy on a polycrystalline sample with a nearly stoichiometric magnetic lattice [2.8(2)% Cr vacancies ...
Quantum magnetism remains a hot topic in condensed matter physics due to its complexity and possible powerful and significant applications in data storage and memory. To understand how the materials can achieve these goals, one should have a clear idea ab ...
This thesis presents the first cavity quantum electrodynamics experiments performed with a degenerate gas of 6Li with strong atom-atom interactions. The first part of this manuscript describes the design and the building of the apparatus that has been e ...
Topological semimetals are frequently discussed as materials platforms for future electronics that exploit the remarkable properties of their quasiparticles. These ideas are mostly based on dispersion relations that mimic relativistic particles, such as We ...
The cascade of electronic phases in CsV3Sb5 raises the prospect to disentangle their mutual interactions in a clean, strongly interacting kagome lattice. When the kagome planes are stacked into a crystal, its electronic dimensionality encodes how much of t ...
The recently synthesized Ag3LiIr2O6 has been proposed as a Kitaev magnet in proximity to the quantum spin liquid phase. We explore its microscopic Hamiltonian and magnetic ground state using many-body quantum chemistry methods and exact diagonalization tec ...
We studied the magnetic excitations in the quasi-one-dimensional (q-1D) ladder subsystem of Sr14-xCaxCu24O41 (SCCO) using Cu L-3-edge resonant inelastic X-ray scattering (RIXS). By comparing momentum-resolved RIXS spectra with high (x = 12.2) and without ( ...
We present a first-principles investigation of the structural, electronic, and magnetic properties of the pristine and Fe-doped alpha-MnO2 using density-functional theory with extended Hubbard functionals. The onsite U and intersite V Hubbard parameters ar ...
