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Potential-induced nanoclustering of metallic catalysts during electrochemical CO2 reduction

Publications associées (30)

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Stability and Degradation Mechanisms of Copper-Based Catalysts for Electrochemical CO2 Reduction

Raffaella Buonsanti, Jan Vávra

To date, copper is the only monometallic catalyst that can electrochemically reduce CO2 into high value and energy-dense products, such as hydrocarbons and alcohols. In recent years, great efforts have been directed towards understanding how its nanoscale ...

Wiley-VCH Verlag GmbH2020

Mapping of Chemical Heterogeneity at Surfaces with High-Throughput Wide-Field Second Harmonic Microscopy

Igor Nahálka

Many industrial processes are based on electrochemical reactions using engineered electrocatalysts. However, the current lack of theoretical knowledge obscures efforts to maximize catalysts' efficiency, and the optimization process is mostly empirical. To ...

EPFL2020

How to polarise an interface with ions: the discrete Helmholtz model

Hubert Girault, Astrid Johana Olaya Avendano, Grégoire Clément Gschwend

The distribution of electrolytes in an electric field usually relies on theories based on the Poisson-Boltzmann formalism. These models predict that, in the case of a metallic electrode, ionic charges screen the electrode potential, leading to concentratio ...

2020

Lithium-Gold Reference Electrode for Potential Stability DuringIn SituElectron Microscopy Studies of Lithium-Ion Batteries

Vasiliki Tileli, Jialiang Fan, Tzu-Hsien Shen, Robin Pierre Alain Girod, Nikolaos Nianias, Jing Hou

Electrochemical liquid-phase transmission electron microscopy (TEM) is showing excellent promise in fundamental studies of energy-related processes including lithium-ion battery (LIB) cycling. A key requirement to accurately interpret the measurements and ...

2020

Imaging the Heterogeneity of the Oxygen Evolution Reaction on Gold Electrodes Operando: Activity is Highly Local

Sylvie Roke, Arianna Marchioro, Igor Nahálka

Understanding the mechanism of the oxygen evolution reaction (OER), the oxidative half of electrolytic water splitting, has proven challenging. Perhaps the largest hurdle has been gaining experimental insight into the active site of the electrocatalyst use ...

2020

Tribocorrosion behaviour of pure titanium in bovine serum albumin solution: A multiscale study

Anna Neus Igual Muñoz

Tribocorrosion behaviour of pure titanium in phosphate buffer saline (PBS) solution has been investigated systematically as a function of surface chemistry and bovine serum albumin (BSA) content in the solution. A ball-on-disk tribometer coupled with an el ...

ELSEVIER2020

Electrosorption at metal surfaces from first principles

Nicola Marzari

Electrosorption of solvated species at metal electrodes is a most fundamental class of processes in interfacial electrochemistry. Here, we use its sensitive dependence on the electric double layer to assess the performance of ab initio thermodynamics appro ...

NATURE PUBLISHING GROUP2020

Fine-Tuning by Triple Bond of Carbazole Derivative Dyes to Obtain High Efficiency for Dye-Sensitized Solar Cells with Copper Electrolyte

Ulf Anders Hagfeldt, Li Zhang

Three novel dyes consisting of a 5,8,15-tris(2-ethylhexyl)-8,15-dihydro-SH-benzo[1,2-b:3,4-b':6,5-b '']tricarbazole (BTC) electron-donating group and a 4,7-bis(4-hexylthiophen-2-yl)benzo[c][1,2,5]thiadiazole (BTBT) pi-bridge with an anchoring group of phen ...

AMER CHEMICAL SOC2020

Sediment replenishment as a measure to enhance river habitats in a residual flow reach downstream of a dam

Anton Schleiss, Mário Jorge Rodrigues Pereira Da Franca, Severin Stähly

Floodplains downstream of a dam, where the natural flow regime is replaced by a constant residual flow discharge, often lack sediment supply and periodic inundation due to the absence of natural flood events. In this study, a flood with a one-year return p ...

Canadian Dam Association2019

Sediment replenishment combined with an artificial flood improves river habitats downstream of a dam

Anton Schleiss, Mário Jorge Rodrigues Pereira Da Franca, Severin Stähly, Christopher Robinson

River reaches downstream dams where a constant residual flow discharge is imposed, often lack sediment supply and periodic inundation due to the absence of natural flood events. In this study, a two-year return flood was released from an upstream reservoir ...

Nature Research2019

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Lithium-Gold Reference Electrode for Potential Stability DuringIn SituElectron Microscopy Studies of Lithium-Ion Batteries

Vasiliki Tileli, Jialiang Fan, Tzu-Hsien Shen, Robin Pierre Alain Girod, Nikolaos Nianias, Jing Hou

2020

Imaging the Heterogeneity of the Oxygen Evolution Reaction on Gold Electrodes Operando: Activity is Highly Local

Sylvie Roke, Arianna Marchioro, Igor Nahálka

2020

Tribocorrosion behaviour of pure titanium in bovine serum albumin solution: A multiscale study

Anna Neus Igual Muñoz

ELSEVIER2020

Fine-Tuning by Triple Bond of Carbazole Derivative Dyes to Obtain High Efficiency for Dye-Sensitized Solar Cells with Copper Electrolyte

Ulf Anders Hagfeldt, Li Zhang

AMER CHEMICAL SOC2020

Sediment replenishment combined with an artificial flood improves river habitats downstream of a dam

Anton Schleiss, Mário Jorge Rodrigues Pereira Da Franca, Severin Stähly, Christopher Robinson

Nature Research2019