Direct observation of non-fully-symmetric coherent optical phonons by femtosecond x-ray diffraction

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Ultrafast Laser Direct-Writing of Self-Organized Microstructures in Ge-Sb-S Chalcogenide Glass

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The structuring of mid-IR materials, such as chalcogenide glass (ChG), at the micro and nano scales, is of high interest for the fabrication of photonic devices in general, and for spectroscopy applications in particular. One efficient method for producing ...

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Ultrashort Pulse Excited Tip-Enhanced Raman Spectroscopy in Molecules

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Vibrational fingerprints of molecules and lowdimension materials can be traced with subnanometer resolution by performing Tip-enhanced Raman spectroscopy (TERS) in a localization of light in the plasmonic nanocavity of the STM enables high spatial resoluti ...

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Ultrafast Photon-Induced Tunneling Microscopy

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Unification of the techniques of ultrafast science and scanning tunneling microscopy (STM) has the potential of tracking electronic motion in molecules simultaneously in real space and real time. Laser pulses can couple to an STM junction either in the wea ...

AMER CHEMICAL SOC2021

Broadband visible two-dimensional spectroscopy of molecular dyes

Majed Chergui, Andre Al Haddad, Lars-Hendrik Mewes, Rebecca Ann Ingle

Two-dimensional Fourier transform spectroscopy is a promising technique to study ultrafast molecular dynamics. Similar to transient absorption spectroscopy, a more complete picture of the dynamics requires broadband laser pulses to observe transient change ...

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The fragmentation mechanism of gold nanoparticles in water under femtosecond laser irradiation

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Plasmonic nanoparticles in aqueous solution have long been known to fragment under irradiation with intense ultrafast laser pulses, creating progeny particles with diameters of a few nanometers. However, the mechanism of this process is still intensely deb ...

2021

Non-classical photon-phonon correlations at room temperature

Santiago Tarrago Velez

With the development of quantum optics, photon correlations acquired a prominent role as a tool to test our understanding of physics, and played a key role in verifying the validity of quantum mechanics. The spatial and temporal correlations in a light fie ...

EPFL2021

Ultrafast-nonlinear ultraviolet pulse modulation in an AlInGaN polariton waveguide operating up to room temperature

Nicolas Grandjean, Jean-François Carlin, Raphaël Butté, Joachim Armand Simonne Ciers, Davide Maria Di Paola

Ultrafast nonlinear photonics enables a host of applications in advanced on-chip spectroscopy and information processing. These rely on a strong intensity dependent (nonlinear) refractive index capable of modulating optical pulses on sub-picosecond timesca ...

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Fundamentals and perspectives of ultrafast photoferroic recording

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The ability to switch ferroics (ferro-, ferri-, antiferromagnets, ferroelectrics, multiferroics) between two stable bit states is one of the keystones of modern data storage technology. Due to many new ideas, originating from fundamental research during th ...

2020

Broadband quasi-phase-matching in dispersion-engineered all-optically poled silicon nitride waveguides

Tobias Kippenberg, Camille Sophie Brès, Rui Ning Wang, Ozan Yakar, Boris Zabelich, Junqiu Liu, Edgars Nitiss

Quasi-phase-matching (QPM) has become one of the most common approaches for increasing the efficiency of nonlinear three-wave mixing processes in integrated photonic circuits. Here, we provide a study of dispersion engineering of QPM second-harmonic (SH) g ...

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Broadband Quasi-Phase-Matching in All-Optically Poled Stoichiometric Silicon Nitride Waveguides

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We show how broadband (>30nm) quasi-phase matching in all-optically poled Si3N4 waveguides provides a platform for efficient sum-frequency generation, and for femtosecond pulse processing such as fcEo detection without the need for group velocity engineeri ...

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