Radioactive decay | EPFL Graph Search

Radioactive decay (also known as nuclear decay, radioactivity, radioactive disintegration, or nuclear disintegration) is the process by which an unstable atomic nucleus loses energy by radiation. A material containing unstable nuclei is considered radioactive. Three of the most common types of decay are alpha, beta, and gamma decay, all of which involve emitting particles. The weak force is the mechanism that is responsible for beta decay, while the other two are governed by the electromagnetism and nuclear force. Radioactive decay is a stochastic (i.e. random) process at the level of single atoms. According to quantum theory, it is impossible to predict when a particular atom will decay, regardless of how long the atom has existed. However, for a significant number of identical atoms, the overall decay rate can be expressed as a decay constant or as half-life. The half-lives of radioactive atoms have a huge range; from nearly instantaneous to far longer than the age of the universe.

CROCUS Concrete Activation Study by γ-ray Spectrometry and TLD Neutron Flux Measurements

Isabelle Tanseri

The semester project was under the course Physics lab IVb at EPFL. At EPFL site, the experimental fission reactor CROCUS is shielded by concrete which becomes radioactive as a result of neutron interaction. The activation is of interest to study for validation of models and cal- culations, and to quantify the amount of radioactive waste when the reactor will be recycled. In this project, measurements on concrete ac- tivation by NaI- and HPGe-detectors were performed on an in-cavity concrete block, together with TLD measurements on neutron flux in- side the core of CROCUS and in the cavity. The concrete activation and neutron flux allows for comparison and validation of models. The in-cavity concrete block had a low activation, trace elements of 60Co and 65Zn seem to be existing. The relative flux was the highest for structures close to the core and at the ceiling. In future projects, more experimental data on both concrete activation and neutron flux would be performed to acquire uncertainty estimations and correction factors.

2017

Submicro- and Nano-Structured Porous Materials for Production of High-Intensity Exotic Radioactive Ion Beams

Sandrina Fernandes

ISOLDE, the CERN Isotope Separator On-line DEvice is a unique source of low energy beams of radioactive isotopes - atomic nuclei that have too many or too few neutrons to be stable. The facility is like a small 'chemical factory', giving the possibility of changing one element to another, by selecting the atomic mass of the required isotope beam in the mass separator, rather as the 'alchemists' once imagined. It produces a total of more than 1000 different isotopes from helium to radium, with half-lives down to milliseconds, by impinging a 1.4 GeV proton beam from the Proton Synchrotron Booster (PSB) onto special targets, yielding a wide variety of atomic fragments. Different components then extract the nuclei and separate them according to mass. The post-accelerator REX (Radioactive beam EXperiment) at ISOLDE accelerates the radioactive beams up to 3 MeV/u for many experiments. A wide international user radioactive ion beam (RIB) community investigates fundamental aspects of nuclear physics, particle and atomic physics, solid-state physics, materials science, astrophysics, biophysics and medicine. However, there are still a number of radioactive isotopes which are not accessible for experimental physics, either because it has been impossible to produce the element of interest, too low yields (number of isotopes per second measured in the beam line) are obtained or due to the higher post-acceleration energies required for the user's experiments. The aim of this thesis was to synthesize oxide and carbide porous materials, to be used as thick targets to increase the intensity of exotic RIBs. This was done by the evaluation of their radioactive isotope release properties and of their stability under irradiation conditions at high temperatures. This thesis is focused on the study of the chemical and physical processes occurring in the target system where the isotopes are produced, before these enter the ion-source system, are mass-separated and are sent to the user beam lines. The products formed in nuclear reactions between a proton beam and the target must, at a first step, diffuse from the interior of the target out to the surface and evaporate from it. Minimum delay times for the diffusion process can be realized by achieving the shortest diffusion lengths of highly-permeable, low-density, open-structure targets and by operating at the highest possible temperature so that release times are minimized and commensurate with the half-life of the isotopes of interest. Whereas until now target materials with micro-scale structures have been synthesized and used for RIB production, new porous submicro- and nano-structured materials offer the advantage of having lower diffusion activation energy of atoms and thus larger diffusion coefficient than the corresponding bulk counterpart, thanks to the increase of surface to volume ratio of these materials. The potential of this phenomenon for isotope mass separation online (ISOL) targets and many other applications is an evident drop of temperature to maintain a fast diffusion process, and higher release efficiency for the production of intense exotic isotope beams. In Chapter 1 the ISOL technique and the RIB production issues are introduced, followed by a review of recent progresses on target materials to increase yield production in the principal existing and next-generation ISOL and In-Flight facilities worldwide. Chapter 2 gives the theoretical fundamentals of diffusion and effusion in solid materials, and addresses specifically diffusion, effusion and release properties of ISOL targets. The study presented in Chapter 3 consists in the evaluation of release properties in different polycrystalline silicon carbide samples. The diffusion coefficients for Be, Na, Mg and F isotopes were extracted from off-line release measurements done at ISOLDE. The full characterization of the release time structure inherent to the physical and chemical processes of the ISOL RIB production on a submicrometric SiC target material (target SiC #334) used at ISOLDE, was made. This last target development resulted in improvement of magnesium short-lived isotopes yields. This was the first demonstration of the successful use of a submicrometric porous material as an ISOL target material, which delivered unprecedented 8x104 21Mg ions per µC. In Chapter 4, the synthesis of porous submicro- and nano-structured alumina to be used as an ISOL target, was followed by materials characterization in terms of microstructure and related with selected isotope release properties. Whenever possible, the release mechanisms were explained or proposed. The approach is relevant for the study of microstructure effects in other solid porous oxide and carbide targets, for optimization of their release performance. Chapter 5 shows the results of the TARPIPE experiment, set up within the design study task of the foreseen ISOL-type European facility called EURISOL, to investigate proton irradiation damage on typical and novel ISOL target materials under continuous proton irradiation at high temperature (> 1273 K). Materials such as SiC, Al2O3, Y2O3, C and Ta in a variety of forms were irradiated at the 72 MeV proton irradiation station of injector 1 at PSI (Paul Scherrer Institute). The effects of radiation damage on these materials were evaluated from microstructure and chemical analyses before and after irradiation by visual inspection, gamma spectroscopy, scanning electronic microscopy and electron dispersive X-ray analysis on a case-by-case basis. The moderate structure evolution of the porous oxide and carbide samples tested confirms that these materials are good candidates for high-power solid targets to be used at the existing and next generation high-power ISOL facilities, such as TRIUMF (TRI-University Meson Facility) and EURISOL (EURopean Isotope Separator On-line). In Chapter 6, the development and testing of a composite high-power alumina target for neon isotope production associated to a cold FEBIAD ion-source exposed to unprecedented proton beam intensities is reported. A 0.5 GeV proton beam from TRIUMF was used up to 25 µA, a factor 10 with respect to the present oxide targets in operation. The yields obtained were compared to the ones delivered by using a 70 µA proton beam in SiC targets at this facility. The target performance in terms of diffusion properties was evaluated. A general conclusion and discussion are given in Chapter 7. The release studies obtained with irradiation and ion implantation techniques on prospective SiC and Al2O3 matrices resulted in the identification of alternative target matrices for fast radioisotope release; this was confirmed experimentally from Na and Mg elements release efficiency determined online for a SiC target. A high-power oxide/metal composite target made of micrometric structural length scale Al2O3 pellets and Nb foils was operated online at unprecedented beam power intensities. Composite targets made of Nb foils and submicro- and nano-structured porous Al2O3 are expected to further increase yields of exotic isotopes. This ISOL target concept can be applied in the future for many other refractory insulating ceramics by using gradient microstructures and/or different ceramic/metallic combinations. Special care has to be taken, in order to minimize the stress induced by a mismatch of the coefficient of thermal expansion in the different ceramic layers and/or the underlying metallic substrate. Micro- and nano-technology fabrication techniques can be used to tailor pore and grain size distribution in ceramic and metallic complex-shaped composite materials and to shape these in compacts, monoliths and fenestrated structures. A balance between large surface area and large macropore volume for optimum target radioisotope release performance must be achieved. The resulting target material must in addition be stable at high temperatures, have good thermo-mechanical resistance and high thermal conductivity under irradiation for long irradiation time. The understanding of isotope release mechanisms in different solid materials, including the porous and dense fast-ion conductors will contribute to the production of exotic RIB at unprecedented high-intensity.

EPFL2010

Measurement of time-dependent CP violation in B0->Dpi decays and optimisation of flavour tagging algorithms at LHCb

Vincenzo Battista

This thesis presents the results of a time-dependent analysis of

B^0\to D^{\mp}\pi^{\pm}

decays using

3~\rm fb^{-1}

of proton-proton collision data collected with the LHCb detector at CERN's Large Hadron Collider during Run 1 with a centre-of-mass energy of

7

(2011) and

8

(2012) TeV. The LHCb experiment is dedicated to the study of the properties of

b

-flavoured hadrons, in particular

CP

violation in the

B

meson system. The Standard Model of Particle Physics describes very precisely the mechanism and the amount of

CP

violation expected in the Universe. However, the observed matter-antimatter asymmetry is larger by several order of magnitude compared to the predictions. This could be explained by the existence of a new source of

CP

violation, originating in New Physics beyond the Standard Model. The time-dependent analysis of

B^0\to D^{\mp}\pi^{\pm}

decays provides constraints on the angle

\gamma

of the Unitarity Triangle, one of the fundamental parameters of the Standard Model related to

CP

violation. Since no sizeable high-order Standard Model processes are expected to contribute, any deviation from the predictions would be an unambiguous signature of New Physics. The current experimental precision on

\gamma

is significantly lower than that of theoretical predictions. This motivates the effort for new experimental determinations of

\gamma

in order to reduce its uncertainty. The analysis of

\Bz\to\Dmp\pipm

decays, although not as sensitive as that obtained from decays of charged

B

mesons into

D^{(*)0}K^{(*)+}

final states, represents an independent and uncorrelated estimation of

\gamma

that contributes to the global combination of all

\gamma

measurements. The result obtained in this thesis is more precise than previous determinations from other experiments (BaBar, Belle) using

B^0\to D^{\mp}\pi^{\pm}

decays. Although based on a very large sample of about half a million signal events, it is still dominated by statistical uncertainties, indicating good prospects for future improvements in precision with more data from Run 2 and beyond. In addition to the

B^0\to D^{\mp}\pi^{\pm}

analysis, this thesis also summarizes the studies to improve the performances of the flavour tagging algorithms used by the LHCb collaboration to infer the flavour of neutral

B

mesons in time-dependent analyses. The performance of these algorithms, being correlated with the kinematics of the reconstructed particles as well as the complexity of the event (number of tracks and primary vertices), showed a significant decrease on Run 2 data (2015--2018), which were collected at a centre-of-mass energy of

13~\rm TeV

. Thanks to new implementations, these algorithms now have a performance similar to that obtained with Run 1 data.

EPFL2018