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An unprecedent asymmetric catalytic benzilic amide rearrangement for the synthesis of a,a-disubstituted piperazinones is reported. The reaction proceeds via a domino [4+1] imidazolidination/formal 1,2-nitrogen shift/1,2-aryl or alkyl migration sequence, em ...
Since the birth of Information Theory, researchers have defined and exploited various information measures, as well as endowed them with operational meanings. Some were born as a "solution to a problem", like Shannon's Entropy and Mutual Information. Other ...
In this paper, we focus on isotropic and stationary sphere-cross-time random fields. We first introduce the class of spherical functional autoregressive-moving average processes (SPHARMA), which extend in a natural way the spherical functional autoregressi ...
The functional linear model extends the notion of linear regression to the case where the response and covariates are iid elements of an infinite-dimensional Hilbert space. The unknown to be estimated is a Hilbert-Schmidt operator, whose inverse is by defi ...
We present a novel framework for the reconstruction of 1D composite signals assumed to be a mixture of two additive components, one sparse and the other smooth, given a finite number of linear measurements. We formulate the reconstruction problem as a cont ...
We revisit the rapid stabilization of the heat equation on the 1-dimensional torus using the backstepping method with a Fredholm transformation. We prove that, under some assumption on the control operator, two scalar controls are necessary and sufficient ...
We present the development of a multiphase adjoint for the Community Multiscale Air Quality (CMAQ) model, a widely used chemical transport model. The adjoint model provides location- and time-specific gradients that can be used in various applications such ...
This thesis work focuses on optimal control of partial differential equations (PDEs) with uncertain parameters, treated as a random variables. In particular, we assume that the random parameters are not observable and look for a deterministic control which ...
Over the past decade we have developed Koopmans functionals, a computationally efficient approach for predicting spectral properties with an orbital-density-dependent functional framework. These functionals impose a generalized piecewise linearity conditio ...
State-of-the-art data analysis tools have to deal with high-dimensional data. Fortunately, the inherent dimensionality of data is often much smaller, as it has an internal structure limiting its degrees of freedom. In most cases, this structure can be appr ...