Mounir Driss Mensi

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High-permeance polymer-functionalized single-layer graphene membranes that surpass the postcombustion carbon capture target

Emad Oveisi, Kumar Varoon Agrawal, Mounir Driss Mensi, Luis Francisco Villalobos Vazquez de la Parra, Shiqi Huang, Guangwei He, Jing Zhao

Membrane-based postcombustion carbon capture can reduce the capture penalty in comparison to absorbent-based separation. To realize this, high-performance membranes are urgently needed with a CO2 permeance exceeding 1000 gas permeation units or GPU, and a ...

2019

Exploring Energy Transfer in a Metal/Perovskite Nanocrystal Antenna to Drive Photocatalysis

Raffaella Buonsanti, Mounir Driss Mensi, Anna Loiudice, Seryio Saris

The use of all-inorganic perovskite nanocrystals (PeNCs) in photocatalytic systems has been limited because of their instability in polar solvents. Encapsulation of PeNCs in inorganic or polymeric matrices has been shown to be effective in overcoming such ...

2019

Retarding Thermal Degradation in Hybrid Perovskites by Ionic Liquid Additives

Mohammad Khaja Nazeeruddin, Paul Joseph Dyson, Zhaofu Fei, Mounir Driss Mensi, Felix Daniel Bobbink, Cristina Roldán Carmona, Zhangjun Huang, Marius Franckevicius, Nikita Drigo, Rui Xia

Recent years have witnessed considerable progress in the development of solar cells based on lead halide perovskite materials. However, their intrinsic instability remains a limitation. In this context, the interplay between the thermal degradation and the ...

2019

Molecular tunability of surface-functionalized metal nanocrystals for selective electrochemical CO2 reduction

Raffaella Buonsanti, Mounir Driss Mensi, James Richard Pankhurst, Yannick Thomas Guntern

Organic ligands are used in homogeneous catalysis to tune the metal center reactivity; in contrast, clean surfaces are usually preferred in heterogeneous catalysis. Herein, we demonstrate the potential of a molecular chemistry approach to develop efficient ...

2019

Synthesis of Cu/CeO2-x Nanocrystalline Heterodimers with Interfacial Active Sites To Promote CO2 Electroreduction

Raffaella Buonsanti, Emad Oveisi, Mounir Driss Mensi, Seyedehbehnaz Varandili, Jan Vávra, Chethana Janardhana Gadiyar, Michal Stanislaw Strach, Jianfeng Huang, Gian Luca De Gregorio

Synergistic effects at metal/metal oxide interfaces often give rise to highly active and selective catalytic motifs. So far, such interactions have been rarely explored to enhance the selectivity in the electrochemical CO2 reduction reaction (CO2RR). Herei ...

2019

Nanocrystal/Metal–Organic Framework Hybrids as Electrocatalytic Platforms for CO2 Conversion

Raffaella Buonsanti, Mounir Driss Mensi, Pascal Alexander Schouwink, Jan Vávra, James Richard Pankhurst, Valeria Mantella, Yannick Thomas Guntern

The tunable chemistry linked to the organic/inorganic components in colloidal nanocrystals (NCs) and metal–organic frameworks (MOFs) offers a rich playground to advance the fundamental understanding of materials design for various applications. Herein, we ...

Wiley-VCH Verlag GmbH2019

Discovery of a self-healing catalyst for the hydrolytic dehydrogenation of ammonia borane

Emad Oveisi, Mounir Driss Mensi, Fatmah Ebrahim, Kyriakos Stylianou, Ngoc Tú Nguyên, Andrzej Gladysiak, Bardiya Valizadeh, Fatma Pelin Uran

Sustainable catalysts based on earth-abundant elements are considered as economical alternatives to precious-metal-bearing catalysts and could be impactful for many applications. Self-healing sustainable catalysts, which in addition to their 'green' charac ...

Royal Society of Chemistry2019

Structural Sensitivities in Bimetallic Catalysts for Electrochemical CO2 Reduction Revealed by Ag-Cu Nanodimers

Raffaella Buonsanti, Emad Oveisi, Mounir Driss Mensi, Valeria Mantella, Jianfeng Huang

Understanding the structural and compositional sensitivities of the electrochemical CO2 reduction reaction (CO2RR) is fundamentally important for developing highly efficient and selective electrocatalysts. Here, we use Ag/Cu nanocrystals to uncover the key ...

2019

Print-Light-Synthesis of Ni and NiFe-nanoscale catalysts for oxygen evolution

Hubert Girault, Emad Oveisi, Mounir Driss Mensi, Andreas Stephan Lesch, Victor Costa Bassetto

By hyphenating inkjet printing and flash light irradiation, Ni- and NiFe-nano-electrocatalysts of diameters below 2.5 nm with ultralow loadings below 2 µg·cm–2 are synthesized. To achieve this, nanoliter ink volumes containing Ni and Fe chlorides as cataly ...

2019

Mixed-phase MOF-derived Titanium Dioxide for Photocatalytic Hydrogen Evolution: The Impact of the Templated Morphology

Emad Oveisi, Mounir Driss Mensi, Pascal Alexander Schouwink, Kyriakos Stylianou, Christopher Patrick Ireland, Bardiya Valizadeh, Stavroula Kampouri

2018

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High-permeance polymer-functionalized single-layer graphene membranes that surpass the postcombustion carbon capture target

Emad Oveisi, Kumar Varoon Agrawal, Mounir Driss Mensi, Luis Francisco Villalobos Vazquez de la Parra, Shiqi Huang, Guangwei He, Jing Zhao

2019