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Influencing the ultrafast plasmon damping time using Fano resonances for nonlinear plasmonics

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Second harmonic generation in glass-based metasurfaces using tailored surface lattice resonances

Olivier Martin, Fabien Sorin, Jérémy Butet, Wei Yan, Dang Tùng Nguyen, Kuang-Yu Yang, Andreas Leber, Chaoqun Dong

Dielectric metasurfaces have shown prominent applications in nonlinear optics due to strong field enhancement and low dissipation losses at the nanoscale. Chalcogenide glasses are one of the promising materials for the observation of nonlinear effects than ...

2021

Nonlinear plasmonics with monocrystalline gold

Sergejs Boroviks

Plasmonic nanostructures allow to controllably enhance linear and nonlinear light-matter interactions by concentrating the electromagnetic fields at the scales below the diffraction limit. This feature is highly desired for many applications, e.g. bio- and ...

2021

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2021

Avalanche multiphoton photoluminescence (AMPL) is observed from coupled Au–Al nanoantennas under intense laser pumping, which shows more than one order of magnitude emission intensity enhancement and distinct spectral features compared with ordinary metall ...

2021

Modes interplay controls the second harmonic generation dynamics of plasmonic nanostructures

Olivier Martin, Andrei Kiselev, Gabriel David Bernasconi

A large amount of experimental and theoretical works deals with the second harmonic generation from different plasmonic geometries. Since they often consider relatively long optical pulses, many of these studies are focused on the investigation of a quasi- ...

SPIE2020

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Second-harmonic generation (SHG) is investigated from three kinds of lithographically fabricated plasmonic systems: Al monomers, Au monomers and Au-Al heterodimers with nanogaps of 20 nm. Spectrally integrated SHG intensities and the linear optical respons ...

2019

Modes interplay and dynamics in the second harmonic generation of plasmonic nanostructures

Olivier Martin, Andrei Kiselev, Gabriel David Bernasconi

The full wave surface integral equation computation of the second harmonic generation (SHG) dynamics for metal spheres and nanorods - presented as multimedia files - is performed to reveal the dynamics of the modes supported by the nanostructure. We demons ...

2019

Plasmonic Metasurfaces to Tailor Second Harmonic Generation

Kuang-Yu Yang

Second harmonic (SH) generation (SHG) in plasmonic nanostructures originates from the surface of centrosymmetric metals where inversion symmetry is broken. The interest in that topic stems from the strong near-field enhancement on the surface of plasmonic ...

EPFL2018

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Due to its symmetry properties, second-harmonic generation in plasmonic nanostructures enables the observation of even-parity modes that couple weakly to the far field. Consequentially, those modes radiate less and thus have a longer lifetime. Using a full ...

SPIE-INT SOC OPTICAL ENGINEERING2018

Less Is More: Enhancement of Second-Harmonic Generation from Metasurfaces by Reduced Nanoparticle Density

Olivier Martin, Jérémy Butet

We investigate optical second-harmonic generation (SHG) from metasurfaces where noncentrosymmetric V-shaped gold nanoparticles are ordered into regular array configurations. In contrast to expectations, a substantial enhancement of the SHG signal is observ ...

2018