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Spin processes and charge dynamics in organic light emitting diodes

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We investigate the spin relaxation of Ho single atom magnets on MgO/Ag(100) as a function of temperature and magnetic field. We find that the spin relaxation is thermally activated at low field, while it remains larger than 1000 s up to 30 K and 8 T. This ...

AMER PHYSICAL SOC2020

Exciton, Biexciton, and Hot Exciton Dynamics in CsPbBr3 Colloidal Nanoplatelets

Jacques-Edouard Moser, Etienne Christophe Socie, Andrés Burgos Caminal, Brener Rodrigo De Carvalho Vale

Lead halide perovskites have emerged as promising materials for light-emitting devices. Here, we report the preparation of colloidal CsPbBr3 nanoplatelets (3 × 4 × 23 nm3) experiencing a strong quasi-one-dimensional quantum confine- ment. Ultrafast transie ...

2020

Exciton-Carrier Dynamics in 2D Perovskites

Jacques-Edouard Moser, Etienne Christophe Socie, Marine Eva Fedora Bouduban, Andrés Burgos Caminal

2D perovskites has become a major topic in the field of perovskite optoelectronics. Here, we aim to unravel the ultrafast dynamics governing the evolution of charge carriers and excitons. We use a combination of ultrabroadband time-resolved THz spectroscop ...

arXiv.org2020

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Two-dimensional Ruddlesden−Popper hybrid lead halide perovskites have become a major topic in perovskite optoelectronics. Here, we aim to unravel the ultrafast dynamics governing the evolution of charge carriers and excitons in these materials. Using a com ...

2020

Nonequilibrium exciton physics in hybrid lead-halide perovskites and anatase titanium dioxide

Tania Palmieri

The strength of the electron-hole interaction in bulk semiconductors is not only determined by the dielectric environment, but also depends on the presence of other quasiparticles - free charge carriers or phonons - that populate the system. In the former ...

EPFL2019

Dynamics of nanoscale systems probed by time-resolved STM-induced luminescence

Anna Maria Roslawska

The efficiency and peculiarities of processes such as surface adsorption or electron-to-photon energy conversion in organic and inorganic structures are determined by the dynamics at the scale of individual molecules, atoms and charges. The timescales of s ...

EPFL2019

From s-polarized, angle-dependent measurements of the electroluminescence spectra in a three-layer phosphorescent organic light-emitting diode, we calculate the exciton distribution inside the 35 nm thick emission layer. The shape of the exciton profile ch ...

2018

Unusually Long-Lived Photocharges in Helical Organic Semiconductor Nanostructures

Jürgen Brugger, Andrzej Sienkiewicz, Holger Frauenrath, Valentin Flauraud, Jan Cornelius Brauer, Liangfei Tian, Thomas Schmaltz, Regina Judith Hafner

Photocharge generation and formation of long-lived charge carriers are relevant in photosynthesis, photocatalysis, photovoltaics, and organic electronics. A better understanding of the factors that determine these processes in synthetic polymer semiconduct ...

AMER CHEMICAL SOC2018

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The electroluminescence of organic films is the central aspect in organic light emitting diodes (OLEDs) and widely used in current display technology. However, its spatial variation on the molecular scale is essentially unexplored. Here, we address this is ...

American Chemical Society2017

Atomic-scale sensing of the magnetic dipolar field from single atoms

Donat Fabian Natterer

Spin resonance provides the high-energy resolution needed to determine biological and material structures by sensing weak magnetic interactions(1). In recent years, there have been notable achievements in detecting(2) and coherently controlling(3-7) indivi ...

Nature Publishing Group2017