Publication

Single-Molecule-Magnet Behavior in Mononuclear Homoleptic Tetrahedral Uranium(III) Complexes

Related publications (63)

Magnetism of Single Surface Adsorbed Atoms Studied with Radio-Frequency STM

This thesis investigates the magnetic properties of single atoms and molecules adsorbed on thin magnesium oxide decoupling layers, grown on a silver single crystal. To address these systems experimentally, we use a low temperature scanning tunneling micros ...

EPFL2024

Long Spin Lifetime in Rare-Earth Single-Atom Magnets at Surfaces

Boris Sorokin

Further miniaturisation of magnetic storage devices requires an advent of new types of magnets, since classical ferromagnetic materials show lack of remanence at nano- and subnanoscale. A single atom can represent the smallest possible bit of information. ...

EPFL2022

Non-exponential magnetic relaxation in magnetic nanoparticles for hyperthermia

Bence Gábor Márkus

Magnetic nanoparticle based hyperthermia emerged as a potential tool for treating malignant tumours. The efficiency of the method relies heavily on the knowledge of magnetic properties of the samples; in particular, knowledge of the frequency dependent com ...

2021

Quantum dynamics in individual surface spins

Tobias Bilgeri

This thesis presents a combined experimental and theoretical study of the classical and quantum magnetization dynamics in single magnetic adatoms and molecules, and on the classical and quantum coherent control thereof. First, a detailed description of the ...

EPFL2021

Scanning SQUID microscopy in a cryogen-free dilution refrigerator

Philip Johannes Walter Moll, Maja Deborah Bachmann

We report a scanning superconducting quantum interference device (SQUID) microscope in a cryogen-free dilution refrigerator with a base temperature at the sample stage of at least 30 mK. The microscope is rigidly mounted to the mixing chamber plate to opti ...

2021

A Magic Angle Spinning Activated O-17 DNP Raser

David Lyndon Emsley, Michael Allan Hope, Snaedis Björgvinsdóttir

In the raser effect, a sample spontaneously emits continuous radiofrequency radiation, allowing exceptionally narrow NMR line widths to be recorded without applying pulses. To achieve this phenomenon, a large negative magnetization must be induced, which w ...

AMER CHEMICAL SOC2021

Coherent Epitaxial Semiconductor-Ferromagnetic Insulator InAs/EuS Interfaces: Band Alignment and Magnetic Structure

Gabriel Aeppli, Vladimir N. Strocov, Sara Marti Sanchez, Yu Liu

Hybrid semiconductor-ferromagnetic insulator heterostructures are interesting due to their tunable electronic transport, self-sustained stray field, and local proximitized magnetic exchange. In this work, we present lattice-matched hybrid epitaxy of semico ...

AMER CHEMICAL SOC2020

Magnetic dynamics across the in-field transition in Ca3Co2O6

Henrik Moodysson Rønnow, Arnaud Magrez, Ivica Zivkovic, Nagabhushan Ganesh Hegde

The discovery of multiple coexisting magnetic phases in the crystallographically homogeneous compound Ca3Co2O6 has stimulated ongoing research activity. In recent years the main focus has been on the zero-field-state properties, where exceedingly long time ...

AMER PHYSICAL SOC2020

Magnetic properties of on-surface synthesized single-ion molecular magnets

Harald Brune, Stefano Rusponi, Marina Pivetta, Jan Gui-Hyon Dreiser, Aparajita Singha, Katharina Johanna Diller

We perform on-surface synthesis of single-ion molecular magnets on an Ag(111) surface and characterize their morphology, chemistry, and magnetism. The first molecule we synthesize is TbPc2 to enable comparison with chemically synthesized and subsequently s ...

2019

Magnetic and structural properties of Ni-substituted magnetoelectric Co4Nb2O9

Henrik Moodysson Rønnow, Ivica Zivkovic, Virgile Yves Favre, Hadi Papi, Hossein Ahmadvand

The magnetic and structural properties of polycrystalline Co4-xNixNb2O9 (x = 1, 2) have been investigated by neutron powder diffraction, magnetization and heat capacity measurements, and density functional theory (DFT) calculations. For x = 1, the compound ...

2019

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