High-Fidelity Determination of Nuclide Inventories for Radioactive Waste Disposal

Valentyn Bykov
EPFL, 2019
EPFL thesis

Abstract

The general license application (RBG) for the Swiss deep geological repository will be submitted in 2024. Furthermore, the decommissioning of the nuclear power plants (NPPs) is coming soon, with the Mühleberg NPP (KKM) scheduled to shut down in 2019. In support of the associated analyses and planning, availability of accurate descriptions of the nuclear waste streams is of paramount importance.

The work described in this thesis represents a significant improvement of Nagra's most important radioactive waste characterization methodologies: for spent fuel, NPP decommissioning waste, and reactor waste. The resulting high-fidelity nuclide inventories will decisively support the future waste disposal research and development, as well as serve the NPP decommissioning planning in general.

The spent fuel characterization demonstrated is based on Polaris. This approach is compared against the code sequence used in the industry (Studsvik CMS), in order to confirm that, when the necessary fuel data is available, either one of these codes can be used to provide detailed nuclide vector for the spent fuel. Afterwards, possible ways to produce the desired nuclide vectors in the future are identified.

For decommissioning waste, every step of the old characterization methodology has been further developed and improved upon. This includes a new, detailed, fully three-dimensional approach to NPP modeling and the development of a new activation sequence (based on the ORIGEN depletion solver), which outputs a highly-resolved component-wise activation distribution and visualization. Additionally, the methodology is extended to apply the method's results for algorithm-optimized packaging concepts and waste volume minimization through decay storage and free release analyses. At the end, recommendations for the future improvements are presented.

The decommissioning waste characterization methodology is then expanded to accommodate reactor waste, and the more complex nature of the non-stationary components of this waste stream (such as the control rods). A systematic general approach, based additionally on the component dose rate measurements, allows for a more efficient and flexible characterization of all reactor waste.

These developments serve as an important foundation in the ongoing transition from a conservative approach towards a best-estimate plus uncertainty (BEPU) waste characterization, which is vital for accurate safety analysis studies, as well as waste and cost minimization.

The results produced by these methodologies will form the basis for the next version of MIRAM (the Swiss Model Inventory of Radioactive Materials), MIRAM2020, which is to be used for the RBG. They will also be used as part of the next Swiss NPP decommissioning cost study, KS2021. At the same time, the obtained results are already being provided to the Swiss NPPs planning their decommissioning, specifically KKM and Beznau (KKB), allowing detailed component-wise segmentation strategies and packaging concepts decision making, finally leading to notable cost reduction for the utilities.

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Valentyn Bykov
EPFL, 2019
EPFL thesis

Abstract

Official source

https://infoscience.epfl.ch/record/264195?ln=en

About this result

Related concepts (15)

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Standardisation des outils de calcul pour les ADS et leur application à différents scénarios de transmutation des déchets

Marco Cometto

The management of radioactive wastes from the nuclear fuel cycle has become an important issue in the development of future, more sustainable nuclear energy systems. Partitioning and transmutation (P&T) of actinides and some long-lived fission products could reduce the mass and radiotoxicity of highlevel wastes and possibly ease repository licensing requirements. Influenced by political and technological developments, an increasing number of countries employing nuclear power have become interested in P&T technology which involves the development of new types of critical and/or sub-critical reactors and very efficient fuel cycle strategies. The present thesis is closely connected to two P&T related projects of the OECD Nuclear Energy Agency in Paris, a numerical benchmark exercise for an accelerator-driven minor actinides burner and a calculational system study on the role of accelerator-driven systems (ADS) and advanced fast reactors (FR) in advanced nuclear fuel cycles. The author co-coordinated the benchmark exercise and performed the comparative analysis of the different "fuel cycle schemes" investigated in the system study. The benchmark exercise contributed to a greater understanding of the physical phenomena characteristic of the transmutation of actinides in a closed fuel cycle, and allowed to test and improve the tools used for modeling ADSs and corresponding advanced fuel cycles. This work thus effectively led to the development of an efficient and more complete calculational scheme, which has permitted an in-depth and reliable analysis of different transmutation scenarios to be carried out. To quantitatively assess the advantages and drawbacks of transmutation, we considered a limited number of "base" transmutation scenarios which constitute an envelope for various possible transmutation strategies employing fast spectrum systems. We then evaluated, for an equilibrium situation, the main aspects which characterise the different transmutation strategies, such as the nuclear park composition, the mass and toxicity of the waste, the need for natural uranium, the in-pile and out-pile mass inventories and, finally, the fuel cycle requirements. Thus, this study has allowed for the reliable comparison of performances of the three main options in the nuclear waste management, viz. open cycle, recycling of plutonium alone and recycling of all the actinides, as well as an evaluation of the advantages and disadvantages of ADSs in comparison to advanced critical reactors in the management of minor actinides or transuranics. The last part of the dissertation is dedicated to a phase-out study for two schemes employing either ADSs or critical reactors. It has been shown thereby that advanced systems, optimised for an equilibrium fuel composition, can indeed be used to reduce the inventory of transuranics. A comparison of ADS and FR performances has been made in this context, and the relative benefits of transmutation have been quantified in each case taking into consideration, more realistically, the residual mass inventory after the shutdown of all nuclear installations.

EPFL2003

During the past ten years, different independent factors, such as the rapidly increasing worldwide demand in energy, societal concerns about greenhouse gas emissions, and the high and volatile prices for fossil fuels, have contributed to the renewed interest in nuclear technology. It is in this context that the Generation IV international forum (GIF) launched the initiative, in 2000, to collaborate on the research and development (R&D) efforts needed for the next generation, i.e. Generation IV, of nuclear reactors. These advanced systems will be ideally deployed beyond the year 2030, following the Generation III or III+ nuclear power plants, which are mainly based on light water technology and are currently entering deployment. A particular goal set for Generation IV systems is closure of the nuclear fuel cycle. Thus, apart from improvements in safety, they are expected to offer a better utilization of natural resources, as also a minimization of long-lived radioactive wastes. Among the systems selected by the GIF, the Gas-cooled Fast Reactor (GFR) is a highly innovative system with advanced fuel geometry and materials (fuel pellets of mixed uranium-plutonium carbide within a plate-type, honeycomb structure made of SiC). It is in the context of the large, 2400 MWth reference GFR design that the present doctoral research has been conducted, the principal aim having been to develop and qualify the control assembly (CA) pattern and corresponding CA implementation scheme for this system. The work has been carried out in three successive and complementary phases: (1) validation of the neutronics tools, (2) the CA pattern development and related static analysis, and (3) dynamic core behavior studies for hypothetical CA driven transients. The deterministic code system ERANOS and its associated nuclear data libraries for fast reactors were developed and validated for the previous generation of sodium-cooled reactors. The validation of ERANOS for GFR applications was, therefore, the first task to be realized in the present research. This has entailed a systematic reanalysis of the GFR-relevant, integral data generated at PSI during the GCFR-PROTEUS experimental program of the 1970's. Thus, during the first phase of the thesis, the reference PROTEUS test lattice from these experiments has been analyzed with ERANOS-2.0 and its associated, adjusted nuclear data library ERALIB1, in order to derive a reference computational scheme to be used later for the GFR analysis. Additionally, benchmark calculations were performed with the Monte Carlo code MCNPX, allowing one to both check the deterministic results and to analyze the sensitivity to different modern data libraries. It has been found that, for the main reaction rate ratios, the new analysis of the GCFR-PROTEUS reference lattice generally yields good agreement – within 1σ measurement uncertainty – with experimental values and with the Monte Carlo simulations. As shown by the analysis, the predictions were in somewhat better agreement in the case of the adjusted ERALIB1 library. The applicability of ERANOS-2.0/ERALIB1 as the reference neutronics tool for the GFR analysis could thus be demonstrated. Furthermore, neutronics aspects related to the novel features of the GFR, for which new experimental investigations are needed, were highlighted. In the second phase of the research, the CA pattern was developed for the GFR, based on iterative neutronics and thermal-hydraulics calculations, 2D and 3D neutronics models for the reactor core having first been set up using the reference ERANOS-2.0/ERALIB1 computational scheme. For the thermal-hydraulics analysis, the CEA code COPERNIC was used. This design work was followed by the study of an appropriate CA implementation scheme (number of CAs and corresponding positions within the core). Detailed neutronics studies revealed the existence of large CA interaction effects, so-called shadowing/anti-shadowing effects leading to an amplification/reduction of the CA worth. The interactions between the absorber pins within a CA, and between the CAs themselves, were investigated in detail, with the goal to optimize the CA efficiency, in terms of the absorber fraction and minimization of the associated heterogeneity effects. The proposed CA pattern consists of 54 absorber pins placed in a triangular lattice. Each absorber pin is a stainless-steel tube filled with highly enriched 10B boron carbide pellets. As a result of the detailed investigations, the absorber pin diameter could be chosen such as to minimize the pin-to-pin influence within the assembly. In particular, a central part of the CA was designed without any absorber pins (zone filled with stagnant helium). A final reduction of the heterogeneity effect (difference between homogeneous and heterogeneous treatments) to 13% was achieved through this feature. Of special importance, the neutronics investigations performed for the reference GFR core ("2004-Core"), especially those related to the CA interactions, have directly contributed to a new core design ("2007-Core"), with the height-to-diameter ratio having been increased to 0.6, compared to 0.3 for the reference core. During the third phase, detailed coupled, 3D neutron-kinetics (NK) and 1D thermal-hydraulics (TH) models were developed for the GFR core, the aim being to arrive at an in-depth understanding of the 3D core behavior during CA driven transients, especially from the viewpoint of spatial effects. The coupled models were developed using the PARCS code for the 3D NK and the TRACE code for the 1D TH modeling. Particular attention was paid to have each individual fuel sub-assembly and CA represented, in order to allow the analysis of local deformations of the 3D distributions of power and safety related parameters, such as the coolant, cladding and fuel temperatures. The validation of the coupled full-core models was performed against reference ERANOS-VARIANT calculations. In particular, the CA worth and reactivity feedbacks were benchmarked, the discrepancies being shown to be relatively low (

EPFL2009

Improvement of the Decay Heat Removal Characteristics of the Generation IV Gas-cooled Fast Reactor

Aaron Simon Epiney

Gas cooling in nuclear power plants (NPPs) has a long history, the corresponding reactor types developed in France, the UK and the US having been thermal neutron-spectrum systems using graphite as the moderator. The majority of NPPs worldwide, however, are currently light water reactors, using ordinary water as both coolant and moderator. These NPPs – of the so-called second generation – will soon need replacement, and a third generation is now being made available, offering increased safety while still based on light water technology. For the longer-term future, viz. beyond the year 2030, R&D is currently ongoing on Generation IV NPPs, aimed at achieving closure of the nuclear fuel cycle, and hence both drastically improved utilization of fuel resources and minimization of long-lived radioactive wastes. Since the very beginning of the international cooperation on Generation IV, viz. the year 2000, the main research interest in Europe as regards the advanced fast-spectrum systems needed for achieving complete fuel cycle closure, has been for the Sodium-cooled Fast Reactor (SFR). However, the Gas-cooled Fast Reactor (GFR) is currently considered as the main back-up solution. Like the SFR, the GFR is an efficient breeder, also able to work as iso-breeder using simply natural uranium as feed and producing waste which is predominantly in the form of fission products. The main drawback of the GFR is the difficulty to evacuate decay heat following a loss-of-coolant accident (LOCA) due to the low thermal inertia of the core, as well as to the low coolant density. The present doctoral research focuses on the improvement of decay heat removal (DHR) for the Generation-IV GFR. The reference GFR system design considered in the thesis is the 2006 CEA concept, with a power of 2400 MWth. The CEA 2006 DHR strategy foresees, in all accidental cases (independent of the system pressure), that the reactor is shut down. For high-pressure events, dedicated DHR loops with blowers and heat exchangers are designed to operate when the power conversion system cannot be used to provide acceptable core temperatures under natural convection conditions. For depressurized events, the strategy relies on a dedicated small containment (called the guard containment) providing an intermediate back-up pressure. The DHR blowers, designed to work under these pressure conditions, need to be powered either by the power grid or by batteries for at least 24 hours. The specific contributions of the present research – aimed at achieving enhanced passivity of the DHR system for the GFR – are design and analysis related to (1) the injection of heavy gas into the primary circuit after a LOCA, to enable natural convection cooling at an intermediate-pressure level, and (2) an autonomous Brayton loop to evacuate decay heat at low primary pressure in case of a loss of the guard-containment pressure. Both these developments reduce the dependence on blower power availability considerably. First, the thermal-hydraulic codes used in the study – TRACE and CATHARE – are validated for gas cooling. The validation includes benchmark comparisons between the codes, serving to identify the sensitivity of the results to the different modeling assumptions. The parameters found to be the most sensitive in this analysis, such as heat transfer and friction models, are then validated via a detailed re-analysis of earlier PSI (EIR, at the time) gas-loop experiments conducted in the 1970s. Conclusions and recommendations on the models to be used for transient analysis are derived. In general, it has been shown that the agreement, between experiments and the correlations for heat transfer and friction used in TRACE and CATHARE, is quite satisfactory. The thus validated codes are then used in the two detailed, DHR improvement studies carried out. The first improvement of the reference DHR strategy is the heavy gas injection. Assuming a DHR blower failure after a LOCA, the helium pressure in the guard containment is not high enough to evacuate the decay heat by natural convection. To improve the natural convection, the effects of injecting different heavy gases (N2, CO2, Ar and a N2/He mixture) into the primary circuit were analyzed, in order to address the possibility of dealing with DHR-blower failure while accepting an intermediate back-up pressure in the guard containment. Furthermore, different injection locations and injection mass flows were considered, and the sensitivity to the number of available DHR loops and LOCA break-sizes was also addressed. It has been found that injecting the heavy gas in the vicinity of the core could lead to overcooling problems. For an injection point sufficiently far from the core, however, both CO2 and N2 are found to be able to cool the core satisfactorily in natural convection. N2 is proposed as the reference, due to possible chemical problems with CO2. The second proposition for DHR improvement is related to the possibility of a simultaneous guard-containment failure, i.e. a loss-of-back-up-pressure (LOBP) combined with a blower failure after a LOCA. In this case the natural convection, even with heavy gas injection, is no longer strong enough to evacuate the decay heat. To address this issue, the possibility of decay heat removal via use of a dedicated autonomous Brayton cycle – as a standalone DHR loop – has been investigated. First, an analytical Brayton cycle model has been set up, so as to identify convenient machine design points and to study the machine's off-design behavior. Two machine designs have then been drawn up: one for helium in order to provide a reference for understanding the Brayton loop behavior in a generic sense, and the other for nitrogen which is the envisaged gas to be injected after a LOCA. Both, the design of the proposed devices and their validation are discussed. Finally, a detailed transient analysis, involving usage of both heavy-gas injection and the Brayton device (i.e. of the complete, proposed DHR system), is presented. This serves to illustrate the effectiveness of the new strategy for the highly hypothetical worst-case scenario of sequential failures following a LOCA.

EPFL2010