Plaquette valence-bond crystal in the frustrated Heisenberg quantum antiferromagnet on the square lattice
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We revisit the SU(6) Heisenberg model on the honeycomb lattice, which has been predicted to be a chiral spin liquid by mean-field theory [G. Szirmai et al., Phys. Rev. A 84, 011611(R) (2011)]. Using exact diagonalizations of finite clusters, infinite proje ...
The study of magnetic frustration has been interesting due to the variety of magnetic ordering observed at low temperatures. At these temperatures thermal fluctuations become redundant and quantum fluctuations play a significant role in the determining the ...
Potassium chromium jarosite, KCr3(OH)(6)(SO4)(2) (Cr-jarosite), is considered a promising candidate to display spin liquid behavior due to the strong magnetic frustration imposed by the crystal structure. However, the ground state magnetic properties have ...
In this thesis I study the synthesis and basic physical properties characterization on 3d, 4d and 5d transition metal compounds. Great success has been obtained in 3d transition metal compounds, in which the electric states are well localized due t ...
Spin systems with strong magnetic interactions might remain disordered avoiding conventional magnetic long-range ordering due to zero-point quantum fluctuations, and supporting a Quantum Spin Liquid (QSL) state. Long-range quantum entanglement in QSLs prom ...
Magnetic properties of AMoOPO4Cl (A=K,Rb) with Mo5+ ions in the 4d1 electronic configuration are investigated by magnetization, heat capacity, and nuclear magnetic resonance (NMR) measurements on single crystals, combined with powder neutron diffraction ex ...
Quantum Monte Carlo simulations provide one of the more powerful and versatile numerical approaches to condensed matter systems. However, their application to frustrated quantum spin models, in all relevant temperature regimes, is hamstrung by the infamous ...
We report electron spin resonance (ESR), Raman scattering, and interband absorption measurements of the multiferroic FeTe2O5Br with two successive magnetic transitions at T-N1 = 11.0 K and T-N2 = 10.5 K. ESR measurements show all characteristics of a low-d ...
Based on high-field 31P nuclear magnetic resonance experiments and accompanying numerical calculations, it is argued that in the frustrated S=1/2 ladder compound BiCu2PO6 a field-induced soliton lattice develops above a critical field of μ0Hc1=20.96(7) T. ...
Collective magnetic excitations are a fascinating aspect of condensed matter physics, where neutron scattering can provide valuable insight into the magnetic properties of physical realisations of model systems. This thesis focuses on the excitation spectr ...