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High-Stable Lead-Free Solar Cells Achieved by Surface Reconstruction of Quasi-2D Tin-Based Perovskites

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A series of novel polymers (P1P6) derived from the combination of different units (including thiophene, triarylamine, and spirobifluorene) were successfully synthesized, completely characterized, and used as hole-transporting materials (HTMs) for perovskit ...

AMER CHEMICAL SOC2019

Phosphonic Acid Modification of the Electron Selective Contact: Interfacial Effects in Perovskite Solar Cells

Wolfgang Richard Tress, Ulf Anders Hagfeldt, Juan-Pablo Correa-Baena, Silver Hamill Turren Cruz, Rebecca Hill

The role electron-transport layers (ETLs) play in perovskite solar cells (PSCs) is still widely debated. Conduction band alignment at the perovskite/ETL interface has been suggested to be an important role for the performance of the solar cells. However, l ...

AMER CHEMICAL SOC2019

Strategic advantages of reactive polyiodide melts for scalable perovskite photovoltaics

Michael Graetzel, Andrey Petrov

Despite tremendous progress in efficiency and stability, perovskite solar cells are still facing the challenge of upscaling. Here we present unique advantages of reactive polyiodide melts for solvent- and adduct-free reactionary fabrication of perovskite f ...

NATURE PUBLISHING GROUP2019

The cost-effective processability and high efficiency of the organic-inorganic metal halide perovskite solar cells (PSCs) have shown tremendous potential to intervene positively in the generation of clean energy. However, prior to an industrial scale-up pr ...

WILEY-V C H VERLAG GMBH2019

Perovskite Solar Cells on the Way to Their Radiative Efficiency Limit - Insights Into a Success Story of High Open-Circuit Voltage and Low Recombination

Wolfgang Richard Tress

Inorganic-organic lead-halide perovskite solar cells have reached efficiencies above 22% within a few years of research. Achieved photovoltages of >1.2 V are outstanding for a material with a bandgap of 1.6 eV - in particular considering that it is solutio ...

Wiley-V C H Verlag Gmbh2017

Investigations on hybrid organic-inorganic perovskites for high performance solar cells

Norman Pellet

Undoubtedly, perovskite solar cells have become a key player in 3rd generation photovoltaics over the last few years. Although it is only in 2012 that the first solid state perovskite solar cell was reported, power conversion efficiencies have increased so ...

EPFL2017

Elucidating the role of chlorine in perovskite solar cells

Gang Wang, Ulf Anders Hagfeldt, Jingshan Luo, Xiaoyu Zhang, Yi Ding, Di Zhang, Li Fan

It has been proposed that introducing the chlorine anion into a CH3NH3PbI3 perovskite material can substantially improve the materials properties as well as the solar cell performance. To elucidate the role of chlorine in perovskite solar cells (PSCs), her ...

Royal Society of Chemistry2017

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Functionalized imidazolium iodide salts (ionic liquids) modified with -CH2-CH=CH2, -CH2C equivalent to CH, or -CH2C equivalent to N groups are applied as dopants in the synthesis of CH3NH3PbI3-type perovskites together with a fumigation step. Notably, a so ...

Wiley-Blackwell2017

We report the presence of defects in CH3NH3PbI3, which is one of the main factors that deteriorates the performance of perovskite solar cells. Although the efficiency of the perovskite solar cells has been improved by curing defects using various methods, ...

Royal Soc Chemistry2017

The presence of voids in perovskite solar cells influences the efficiency because of accelerated charge recombination. The induced electric field near voids due to band bending attracts photogenerated electrons and holes toward the voids, leading to carrie ...

Amer Chemical Soc2017