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The subject of the present work is discovery and in-depth characterization of a new class of functional materials. Tuning of the bond polarity and orbital occupation with a goal of establishing balance between localization and delocalization of electrons - ...
The dynamics of the S = 3/2 kagome antiferromagnet chromium jarosite, KCr3(OD)(6)(SO4)(2), was studied using high-resolution neutron time-of-flight spectroscopy on a polycrystalline sample with a nearly stoichiometric magnetic lattice [2.8(2)% Cr vacancies ...
Bound-states of particles are an interesting problem in quantum mechanics dating back to 1931 Bethe's solution of spin-1/2 Heisenberg chain. These exotic composite states are realized in quantum magnets and are detectable in inelastic neutron scattering (I ...
Autoregressive Neural Networks (ARNNs) have shown exceptional results in generation tasks across image, language, and scientific domains. Despite their success, ARNN architectures often operate as black boxes without a clear connection to underlying physic ...
Quantum spin liquids are highly entangled magnetic states with exotic properties. The S = 1/2 square-lattice Heisenberg model is one of the foundational models in frustrated magnetism with a predicted, but never observed, quantum spin liquid state. Isostru ...
We report neutron scattering measurements on YbMnSb2 which shed light on the nature of the magnetic moments and their interaction with Dirac fermions. Using half-polarized neutron diffraction we measured the field-induced magnetization distribution in the ...
In spin systems, geometrical frustration describes the impossibility of minimizing simultaneously all the interactions in a Hamiltonian, often giving rise to macroscopic ground-state degeneracies and emergent low-temperature physics. In this thesis, combin ...
The magnetic propertiesof transition-metal ions aregenerallydescribed by the atomic spins of the ions and their exchange coupling.The orbital moment, usually largely quenched due the ligand field,is then seen as a perturbation. In such a scheme, S = 1/2 io ...
In this paper we study a fully connected planted spin glass named the planted XY model. Motivation for studying this system comes both from the spin glass field and the one of statistical inference where it models the angular synchronization problem. We d ...
Recent neutron-diffraction experiments in honeycomb CrI3 quasi-2D ferromagnets have evinced the existence of a gap at the Dirac point in their spin-wave spectra. The existence of this gap has been attributed to strong in-plane Dzyaloshinskii-Moriya or Kita ...