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The article describes the use of neutron scattering methods (including powder diffraction, vibrational and rotational spectroscopy, and quasi-elastic scattering) to enhance our understanding of the performance (or lack of performance) of novel storage and ...
This work presents a new, field-deployable technique for continuous, high-resolution measurements of methane mixing ratios from ice cores. The technique is based on a continuous flow analysis system, where ice core samples cut along the long axis of an ice ...
Extent-based incremental identification uses the concept of extents and the integral method of parameter estimation to identify reaction kinetics from concentration measurements. The approach is rather general and can be applied to open both homogeneous an ...
In relation to Arctic warming, the possible occurrence of methane hydrate degassing events has attracted an increasing interest in recent years. We evaluate the atmospheric impact of rapid and massive emissions of methane and how they are imprinted in ice ...
Unique worldwide, Lake Kivu stores enormous amounts of CH4 and CO2. A recent study reported that CH4 concentrations in the lake have increased by up to 15% in the last 30 years and that accumulation at this rate could lead to catastrophic outgassing by sim ...
Tropical reservoirs have been identified as important methane (CH4) sources to the atmosphere, primarily through turbine and downstream degassing. However, the importance of ebullition (gas bubbling) remains unclear. We hypothesized that ebullition is a di ...
The oxygen-isotope records from Greenland ice cores show a very strong, reproducible pattern of alternation between warm Greenland Interstadials (GI) and cold Greenland Stadials (GS) at millennial-scale during the last glacial period. Here we summarise wha ...
We compare a variety of methods for estimating the gas/ice depth offset (Δdepth) at EPICA Dome C (EDC, East Antarctica). (1) Purely based on modelling efforts, Δdepth can be estimated combining a firn densification with an ice flow model. (2) The diffusive ...
Global measurements of atmospheric methane (CH4) concentrations continue to show large interannual variability whose origin is only partly understood. Here we quantify the influence of the El Nino-Southern Oscillation (ENSO) on wetland CH4 emissions, which ...
The Hudson Bay Lowlands (HBL) is the second largest boreal wetland ecosystem in the world and an important natural source of global atmospheric methane. We quantify the HBL methane emissions by using the GEOS-Chem chemical transport model to simulate aircr ...
