Résonance paramagnétique électronique

Science de la nature
Chimie
Chimie physique
Spectroscopie

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Antiferromagnetic resonance in TmFeO3 at high temperatures

Jean-Philippe Ansermet, Arnaud Magrez, Haiming Yu, Marcin Bialek

Temperature dependence of the antiferromagnetic resonance spectrum in a thulium orthoferrite (TmFeO3) poly-crystalline sample was studied by transmission spectroscopy in the frequency range of 0.1–0.75 THz and temperature range of 300–670 K, up to its Néel ...

2020

Enhanced Intersystem Crossing and Transient Electron Spin Polarization in a Photoexcited Pentacene–Trityl Radical

David Lyndon Emsley, Jacques-Edouard Moser, Aaron James Rossini, Dominik Józef Kubicki, Moreno Lelli, Etienne Christophe Socie, Gabriele Stevanato, Claudia Esther Avalos

Identifying and characterizing systems that generate well-defined states with large electron spin polarization is of high interest for applications in molecular spintronics, high-energy physics, and magnetic resonance spectroscopy. The generation of electr ...

2020

Magnetic resonance spectroscopy (MRS) and spectroscopic imaging (MRSI) allow the chemical analysis of physiological processes in vivo and provide powerful tools in the life sciences and for clinical diagnostics. Excellent homogeneity of the static B(0)magn ...

2020

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SA-BDPA is a water-soluble, narrow-line width radical previously used for dynamic nuclear polarization (DNP) signal enhancement in solid-state magic angle spinning NMR spectroscopy. Here, we report the first study using SA-BDPA under dissolution DNP condit ...

AMER CHEMICAL SOC2020

Fabrication of clamped-clamped beam resonators with embedded fluidic nanochannel

Philippe Renaud, Luis Guillermo Villanueva Torrijo, Annalisa De Pastina, Damien Maillard, Stefano Silvio Giovanni Varricchio, Carlo Ricciardi, Davide Scaiola, Stefano Stassi

Suspended nanochannel resonators (SNRs) are promising devices able to characterize mass down to the attogram scale, thus being able to detect nanoparticles or biomolecules. In this paper, we present a flexible fabrication process for SNRs based on a sacrif ...

ELSEVIER2020

UV-Irradiated 2-Keto-(1-C-13)Isocaproic Acid for High-Performance C-13 Hyperpolarized MR

Andrea Capozzi, Arthur César Pinon

Enhancing the sensitivity of magnetic resonance spectroscopy/imaging (MRS/MRI) by dissolution dynamic nuclear polarization (dDNP) has expanded the scope of MRS applications to new fields of research. Most importantly, it has paved the way toward noninvasiv ...

AMER CHEMICAL SOC2020

Spin-wave coupling to electromagnetic cavity fields in dysposium ferrite

Jean-Philippe Ansermet, Arnaud Magrez, Marcin Bialek

Coupling of spin waves with electromagnetic cavity field is demonstrated in an antiferromagnet, dysprosium ferrite (DyFeO3). By measuring transmission at 0.2-0.35 THz and sweeping sample temperature, magnon-photon coupling signatures were found at crossing ...

AMER PHYSICAL SOC2020

From synchrotrons for XFELs: the soft x-ray near-edge spectrum of the ESCA molecule

Christoph Bostedt

A predictive understanding of soft x-ray near-edge absorption spectra of small molecules is an enduring theoretical challenge and of current interest for x-ray probes of molecular dynamics. We report the experimental absorption spectrum for the electron sp ...

2020

Liquid-phase hydrodeoxygenation of phenol over silica-supported MoOx-ReOx catalysts was investigated at 300 degrees C and 5 MPa of H-2. Mixed-oxides catalysts with similar surface metal density (2.3 atoms of metal per nm(2) of SiO2) but different relative ...

2020

Temperature dependence of reconfigurable bandstop filters using vanadium dioxide switches

Mihai Adrian Ionescu, Matteo Cavalieri, Andrei Müller

In this Letter, we report and investigate the temperature dependency of various radio frequency (RF) parameters for a fabricated reconfigurable bandstop filter with vanadium dioxide (VO2) switches measured up to 55 GHz. Here, the insulator-to-metal (ITM) a ...

2020

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