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Multiphoton spectroscopy of monodeuterated water is employed to determine more than 210 new energy levels of HDO in the 25 000–35 000 cm region. These new empirical energy levels are used to fit a potential energy surface (PES) valid between 20 000 cm and ...
2021
In spin systems, geometrical frustration describes the impossibility of minimizing simultaneously all the interactions in a Hamiltonian, often giving rise to macroscopic ground-state degeneracies and emergent low-temperature physics. In this thesis, combin ...
A magnetic impurity is placed on the tip of a scanning tunnelling microscope, allowing direct tunnelling between two Yu-Shiba-Rusinov bound states. This technique can probe and enhance the impurity state lifetime. There is a limit to the miniaturization of ...
2020
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Single lanthanide atoms and molecules are promising candidates for atomic data storage and quantum logic due to the long lifetime of their magnetic quantum states. Accessing and controlling these states through electrical transport requires precise knowled ...
We theoretically investigate the electron transport in armchair and zigzag graphene nanoribbons (GNRs) chemically functionalized withp-polyphenyl and polyacene groups of increasing length. Our nearest-neighbor tight-binding calculations indicate that, depe ...
Two-dimensional systems with C2T (PT) symmetry exhibit the Euler class topology E is an element of Z in each two-band subspace realizing a fragile topology beyond the symmetry indicators. By systematically studying the energy levels of Euler insulating pha ...
We study the asymptotic behavior of the N-clock model, a nearest neighbors ferromagnetic spin model on the d-dimensional cubic epsilon-lattice in which the spin field is constrained to take values in a discretization S-N of the unit circle S-1 consisting o ...
2021
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Determination of the three-dimensional atomic-level structure of powdered solids is one of the key goals in current chemistry. Solid-state NMR chemical shifts can be used to solve this problem, but they are limited by the high computational cost associated ...
AMER CHEMICAL SOC2022
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Eigenmode coalescence imparts remarkable properties to non-Hermitian time evolution, culminating in a purely non-Hermitian spectral degeneracy known as an exceptional point (EP). Here, we revisit time evolution around EPs, looking at both static and period ...
The under-coordinated defects within perovskite and its relevant interfaces always attract and trap the free carriers via the electrostatic force, significantly limiting the charge extraction efficiency and the intrinsic stability of perovskite solar cells ...
