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We present a review of wave packet dynamics in different systems and stress their relation to information on the ultrafast structural changes. We show how dynamical information is obtained from ultrafast optical pump-probe studies on structural changes in ...
Recording of gratings by interference of two pump pulses and diffraction of a third probe pulse is useful for investigating ultrafast material phenomena. We demonstrate, in theory and experiment, that the temporal resolution in such configurations does not ...
Spatial gratings are recorded holographically by two femtosecond pump pulses at 388 nm in lithium niobate (LiNbO3) crystals and read out by a Bragg-matched, temporally delayed probe pulse at 776 nm. We claim, to our knowledge, the first holographic pump-pr ...
In 2-color optical Kerr effect measurements of water, addnl. signals can occur in the pulse overlap region if the energy difference between pump and probe pulses approaches the Raman resonance of the OH-stretch vibration. These features can be understood b ...
The formation and quenching of the triplet state of xanthone are studied by femtosecond techniques. As revealed by femtosecond fluorescence spectroscopy, the primarily excited 1ππ* state decays within 1.5 ps. In a transient absorption experiment, this time ...
Femtosecond pump pulses are strongly attenuated in lithium niobate owing to two-photon absorption; the relevant nonlinear coefficient beta(p) ranges from similar to 3.5 cm/GW for lambda(p) = 388 nm to similar to 0.1 cm/GW for 514 nm. In collinear pump-prob ...
We have observed the filamentation of optical pulses in carbon disulfide(CS2) using femtosecond time-resolved optical polarigraphy(FTOP)1. A pump-probe setup is used to capture the propagation of a 150 femtosecond laser pulse in CS2. The probe pulse propag ...
The dynamics of electron bubble formation upon excitation of the A(3ss) Rydberg orbital of NO in solid Ne was studied by conventional spectroscopy and fs pump-probe spectroscopy. The fs pump pulse initiates the formation of a bubble by the expansion of the ...
The propagation of high-power femtosecond light pulses in lithium niobate crystals (LiNbO3) is investigated experimentally and theoretically in collinear pump-probe transmission experiments. It is found within a wide intensity range that a strong decrease ...
In this work we present the coherent control of polariton parametric scattering with weak phase locked probe pulses. It is demonstrated that the signal emission arising from the parametric scattering is completely coherent for moderate excitation power, wh ...
