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Chlorine dioxide (ClO2) decay in the presence of typical metal oxides occurring in distribution systems was investigated. Metal oxides generally enhanced ClO2 decay in a second-order process via three pathways: (1) catalytic disproportionation with equimol ...
The aim of the present thesis is to investigate several aspects of: the proteins mechanics, interprotein interactions and to study also new techniques, theoretical and technical, to obtain and analyze the force spectroscopy experiments. The first section i ...
Reaction rate distribution measurements are reported from experiments in an SCWR-like test lattice performed with separated moderator and coolant regions. This work was done at the zero-power research reactor PROTEUS at the Paul Scherrer Institute in Switz ...
LiBH4 contains 18.5 wt% hydrogen and undergoes a structural phase transition (orthorhombic → hexagonal) at 381 K which is associated with a large increase in hydrogen and lithium solid-state mobility. We investigated the hydrogen dynamics in the low temper ...
Coordinating component behaviour and, in particular, concurrent access to resources is among the key difficulties of building large concurrent systems. To address this, developers must be able to manipulate high-level concepts, such as Finite State Machine ...
The enhancement of fluorescence and Raman scattering by plasmonic nanostructures is studied theoretically with special focus on the effects of the observed molecule's properties and the realistic geometry of the plasmonic nanostructure. Numerical experimen ...
Density functional calculations applying periodic boundary conditions have been performed to investigate adsorption and cracking of light alkanes (C 3-C 6) on zeolite H-ZSM-5. Intrinsic energy barriers were obtained from single-point calculations by applyi ...
In this thesis, I describe the design and first applications of a new molecular-beam/surface-science ultra-high vacuum apparatus. The new machine combines rovibrational state-selective infrared pumping of gas-phase reactants with reflection absorption infr ...
Let r : S x S -> R+ be the jump rates of an irreducible random walk on a finite set S, reversible with respect to some probability measure m. For alpha > 1, let g : N -> R+ be given by g(0) = 0, g(1) = 1, g(k) = (k/k - 1)(alpha), k >= 2. Consider a zero ra ...
We report the design and characterization of a new molecular-beam/surface-science apparatus for quantum state-resolved studies of gas/surface reaction dynamics combining optical state-specific reactant preparation in a molecular beam by rapid adiabatic pas ...
