Publications de Michael Graf | EPFL Graph Search

Electrochemical Functionalization of Selectively Addressed MoS2 Nanoribbons for Sensor Device Fabrication

Aleksandra Radenovic, Vasiliki Tileli, Martina Lihter, Michael Graf, Michal Daniel Macha, Yanfei Zhao, Tzu-Hsien Shen, Miao Zhang

Tailoring the surface properties of 2D materials, such as transition metal dichalcogenides (TMDCs), at the nanoscale is becoming essential in the fabrication of various 2D material-based nanoelectronic devices. Due to the chemical inertness of their basal ...

AMER CHEMICAL SOC2021

Microscopic Detection Analysis of Single Molecules in MoS2 Membrane Nanopores

Aleksandra Radenovic, Michael Graf

A systematic microscopic analysis of the various resistive effects involved in the electronic detection of single biomolecules in a nanopore of a MoS2 nanoribbon is presented. The variations of the transverse electronic current along the two-dimensional (2 ...

2020

Wafer-Scale Fabrication of Nanopore Devices for Single-Molecule DNA Biosensing using MoS2

Aleksandra Radenovic, Andras Kis, Martina Lihter, Mukesh Kumar Tripathi, Mukeshchand Thakur, Andrey Chernev, Michael Graf, Michal Daniel Macha, Jochem Deen

Atomically thin (2D) nanoporous membranes are an excellent platform for a broad scope of academic research. Their thickness and intrinsic ion selectivity (demonstrated for example in molybdenum disulfide-MoS2) make them particularly attractive for single-m ...

2020

Light-Enhanced Blue Energy Generation Using MoS2 Nanopores

Aleksandra Radenovic, Andras Kis, Martina Lihter, Michael Graf, Dmitrii Unuchek, Aditya Sarathy

Blue energy relies on the chemical potential difference between solutions of high and low ionic concentrations, potentially providing an independent energy source at estuaries around the world. The energy conversion relies on reverse electrodialysis via io ...

2019

Fabrication and practical applications of molybdenum disulfide nanopores

Aleksandra Radenovic, Martina Lihter, Mukeshchand Thakur, Michael Graf, Ke Liu, Jiandong Feng

Among the different developed solid-state nanopores, nanopores constructed in a monolayer of molybdenum disulfide (MoS2) stand out as powerful devices for single-molecule analysis or osmotic power generation. Because the ionic current through a nanopore is ...

2019

Nanoscale Selective Passivation of Electrodes Contacting a 2D Semiconductor

Aleksandra Radenovic, Martina Lihter, Michael Graf

2D semiconducting materials have become the central component of various nanoelectronic devices and sensors. For sensors operating in liquid, it is crucial to efficiently block the electron transfer that occurs between the electrodes contacting the 2D mate ...

2019

2D nanopores: fabrication, energy harvesting and field-effect sensing

Michael Graf

Solid-state nanopores are man-made, nano-sized openings in membranes separating two chambers containing an electrolyte solution. When applying an electric field across the membrane, the nanopore provides the only path for mobile ions to pass from one side ...

EPFL2019

Transverse Detection of DNA Using a MoS2 Nanopore

Aleksandra Radenovic, Martina Lihter, Michael Graf, Sanjin Marion

Classical nanopore sensing relies on the measurement of the ion current passing through a nanopore. Whenever a molecule electrophoretically translocates through the narrow constriction, it modulates the ion current. Although this approach allows one to mea ...

2019

Orthogonal Tip-to-Tip Nanocapillary Alignment Allows for Easy Detection of Fluorescent Emitters in Femtomolar Concentrations

Aleksandra Radenovic, Michael Graf, Po-Ling Chang

Here we present the realization of a novel fluorescence detection method based on the electromigration of fluorescent molecules within a nanocapillary combined with the laser excitation through a platinum (Pt)-coated nanocapillary. By using the Pt nanocapi ...

American Chemical Society (ACS)2018

Transverse Detection of DNA in a MoS2 Nanopore

Aleksandra Radenovic, Michael Graf, Ke Liu, Aditya Sarathy

2018