Personne

Christoph Bostedt

Publications associées (27)

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Electronic Population Transfer via Impulsive Stimulated X-Ray Raman Scattering with Attosecond Soft-X-Ray Pulses

Christoph Bostedt, Xiang Li, Andre Al Haddad, Solène Oberli, Siqi Li

Free-electron lasers provide a source of x-ray pulses short enough and intense enough to drive nonlinearities in molecular systems. Impulsive interactions driven by these x-ray pulses provide a way to create and probe valence electron motions with high tem ...

AMER PHYSICAL SOC2020

Characterizing crystalline defects in single nanoparticles from angular correlations of single-shot diffracted X-rays

Christoph Bostedt, Alessandro Colombo, Giorgio Rossi

Characterizing and controlling the uniformity of nanoparticles is crucial for their application in science and technology because crystalline defects in the nanoparticles strongly affect their unique properties. Recently, ultra-short and ultra-bright X-ray ...

INT UNION CRYSTALLOGRAPHY2020

Intense x-ray free-electron laser (XFEL) pulses hold great promise for imaging function in nanoscale and biological systems with atomic resolution. So far, however, the spatial resolution obtained from single shot experiments lags averaging static experime ...

2020

Angular Momentum in Rotating Superfluid Droplets

Christoph Bostedt, Camila Bacellar Cases Da Silveira

The angular momentum of rotating superfluid droplets originates from quantized vortices and capillary waves, the interplay between which remains to be uncovered. Here, the rotation of isolated submicrometer superfluid He-4 droplets is studied by ultrafast ...

AMER PHYSICAL SOC2020

Imaging plasma formation in isolated nanoparticles with ultrafast resonant scattering

Christoph Bostedt, Daniela Rupp, Alessandro Colombo

We have recorded the diffraction patterns from individual xenon clusters irradiated with intense extreme ultraviolet pulses to investigate the influence of light-induced electronic changes on the scattering response. The clusters were irradiated with short ...

2020

Previous single-pulse extreme ultraviolet and x-ray coherent diffraction studies revealed that superfluid He-4 droplets obtained in a free jet expansion acquire sizable angular momentum, resulting in significant centrifugal distortion. Similar experiments ...

AMER PHYSICAL SOC2020

Formamide, a simple model bio-molecule (HCONH2), is irradiated with high intensity, ultrashort pulses from an x-ray free electron laser. Ionic fragments resulting from photoionization and subsequent decay processes are recorded, as well as the electronic s ...

2020

Characterizing crystalline defects in single Xe nanoparticles from angular correlations of single-shot diffracted X-rays

Yiming Li, Christoph Bostedt

We performed a wide-angle X-ray scattering experiment of single Xe nanoparticles using an X-ray free electron laser. We developed a novel analysis method that focuses on the angular correlation between plural Bragg spots in single-shot diffraction patterns ...

IOP PUBLISHING LTD2020

A predictive understanding of soft x-ray near-edge absorption spectra of small molecules is an enduring theoretical challenge and of current interest for x-ray probes of molecular dynamics. We report the experimental absorption spectrum for the electron sp ...

2020

X-ray free-electron lasers (XFELs) deliver ultrashort coherent laser pulses in the X-ray spectral regime, enabling novel investigations into the structure of individual nanoscale samples. In this work, we demonstrate how single-shot small-angle X-ray scatt ...

2019