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The modification of glass nanopipettes with polyethyleneimines (PEIs) has been successfully achieved by a relatively simple method, and the smallest tip opening is around 3 nm. Thus, in a much wider range of glass pipettes with radii from several nanometers to a few micrometers, the ion current rectification (ICR) phenomenon has been observed. The influences of different KCl concentrations, pH values, and tip radii on the ICR are investigated in detail. The sizes of PEIs have been determined by dynamic light scattering, and the effect of the sizes of PEIs for the modification, especially for a few nanometer-pipettes in radii, is also discussed. These findings systemically confirm and complement the theoretical model(7,18) and provide a platform for possible selectively molecular detection and mimic biological ion channels.
Athanasios Nenes, Qianyu Zhao, Yan Feng, Haofei Yu
Jian Wang, Matthias Finger, Lesya Shchutska, Qian Wang, Matthias Wolf, Varun Sharma, Konstantin Androsov, Jan Steggemann, Leonardo Cristella, Xin Chen, Davide Di Croce, Mingkui Wang, Zhirui Xu, João Miguel das Neves Duarte, Tagir Aushev, Tian Cheng, Yixing Chen, Werner Lustermann, Andromachi Tsirou, Alexis Kalogeropoulos, Andrea Rizzi, Ioannis Papadopoulos, Paolo Ronchese, Thomas Muller, Ho Ling Li, Giuseppe Codispoti, Hua Zhang, Siyuan Wang, Peter Hansen, Daniel Gonzalez, Tao Huang, David Vannerom, Michele Bianco, Kun Shi, Wei Shi, Abhisek Datta, Ji Hyun Kim, Donghyun Kim, Dipanwita Dutta, Zheng Wang, Sanjeev Kumar, Wei Li, Yong Yang, Geng Chen, Yi Wang, Ajay Kumar, Ashish Sharma, Georgios Anagnostou, Joao Varela, Csaba Hajdu, Muhammad Ahmad, Ekaterina Kuznetsova, Ioannis Evangelou, Matthias Weber, Muhammad Shoaib, Milos Dordevic, Vineet Kumar, Vladimir Petrov, Francesco Fiori, Quentin Python, Meng Xiao, Hao Liu, Sourav Sen, Yanlin Liu, Viktor Khristenko, Marco Trovato, Gurpreet Singh, Fan Xia, Xiao Wang, Bibhuprasad Mahakud, Jing Li, Rajat Gupta, Zhen Liu, Lei Feng, Muhammad Waqas, Hui Wang, Seungkyu Ha, Davide Cieri, Maren Tabea Meinhard, Giorgia Rauco, Ali Harb, Benjamin William Allen, Long Wang, Pratyush Das, Miao Hu, Lei Li