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State-to-state scattering of CH₄ from Ni(111) and Gr/Ni(111)

Publications associées (149)

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Toward Wearable Biosensing by Spectroscopy-free Raman Shift Detection and Soft Optofluidics

Ata Jedari Golparvar

This thesis introduces spectroscopy-free Raman biosensing, which may find increasing use in the next generation of wearable devices for preventive healthcare. While wearables have made substantial advancements in detecting physical biomarkers, they have ye ...

EPFL2024

Quantum state-resolved methane scattering from Ni(111) and NiO(111) by bolometer infrared laser tagging: The effect of surface oxidation

Rainer Beck, Christopher Scott Reilly, Bo-Jung Chen, Patrick Floss

We describe a novel UHV state-to-state molecule/surface scattering apparatus with quan- tum state preparation of the incident molecular beam and angle-resolved quantum state detection of the scattered molecules. State resolved detection is accomplished usi ...

2023

Surface-induced vibrational energy redistribution in methane/surface scattering depends on catalytic activity

Rainer Beck, Christopher Scott Reilly, Patrick Floss

Recent state-to-state experiments of methane scattering from Ni(111) and graphene-covered Ni(111) combined with quantum mechanical simulations suggest an intriguing correlation between the surface-induced vibrational energy redistribution (SIVR) during the ...

2023

Linear scattering theory of short-pulse reflectometry

Stefano Coda, Stephan Brunner, Oleg Krutkin

The linear scattering theory of short pulse reflectometry is presented. An expression for the scattering signal is obtained by applying the perturbation theory approach for solving the Helmholtz equation. Based on these analytical results, a method for mea ...

2023

Kinetics of information scrambling in correlated metals: Disorder-driven transition from shock wave to Fisher or Kolmogorov-Petrovsky-Piskunov dynamics

Camille Didier Georges Aron

Quenched disorder slows down the scrambling of quantum information. Using a bottom-up approach, we formulate a kinetic theory of scrambling in a correlated metal near a superconducting transition, following the scrambling dynamics as the impurity scatterin ...

College Pk2023

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A leading nonlinear effect in magnonics is the interaction that splits a high-frequency magnon into two low-frequency magnons with conserved linear momentum. Here, we report experimental observation of nonlocal three-magnon scattering between spatially sep ...

AMER PHYSICAL SOC2023

State-to-state surface scattering of methane studied by bolometric infrared laser tagging detection

Bo-Jung Chen

State-to-state molecule/surface scattering experiments prepare the incident molecules in a specific quantum state and measure the quantum state distribution of the scattered molecules. The comparison of state resolved experiments with theory can serve as s ...

EPFL2022

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3D printing has revolutionized the manufacturing of volumetric components and structures in many areas. Several fully volumetric light-based techniques have been recently developed thanks to the advent of photocurable resins, promising to reach unprecedent ...

WILEY2022

We give a broad overview of the historical development and physics of Brillouin scattering. We discuss the seminal papers of Brillouin and Mandelstam and give the historical context of their research. We discuss the development of experiments and observati ...

Elsevier2022

We report a state-prepared, state-resolved study of rotational scattering of a diatomic molecule from a solid surface. Specifically, H-2 molecules with 80 meV kinetic energy are rotationally aligned in the j = 3 rotational state via stimulated Raman pumpin ...

AIP Publishing2021