Femtosecond dynamics of electronic 'bubbles' in solid argon: viewing the inertial response and the bath coherences
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This thesis reports on results of three different experiments of photo-induced structural dynamics in the condensed phase, investigated by time-resolved pump-probe spectroscopy with femtosecond time-resolution. In the first part, we address the ultrafast d ...
Four studies investigated the reliability and validity of thin slices of nonverbal behavior from social interactions including (a) how well individual slices of a given behavior predict other slices in the same interaction; (b) how well a slice of a given ...
A complete characterization, based on fs pump-probe spectroscopy and mol. dynamics simulations, is presented of the ultrafast dynamics of electronic bubble formation in solid para-H2 upon impulsive excitation of impurity-doped sites, which correlate with t ...
In this work we present the implantable and wearable measurement system developed for smart knee prostheses monitoring. The kinematic measurement system contains three anisotropic magnetoresistive sensors embedded into the polyethylene part of the prosthes ...
Time-resolved photoelectron spectroscopy can obtain detailed information about the dynamics of a chemical process on the femtosecond timescale. The resulting signal from such detailed experiments is often difficult to analyze and therefore theoretical calc ...
The excitation of the Rydberg states is used to study the nonpolar solvation dynamics in supercrit. fluids (SCFs). The system NO in supercrit. Ar serves as the model system. First, the steady-state, absorption and fluorescence spectra of the NO X 2P-A 2S+( ...
Mol.-dynamics simulations of structural relaxation in electronically excited NO-doped solid neon are presented. The NO impurity is excited to its lowest A (3ss) Rydberg state, inducing a rearrangement of the surrounding medium in the form of a bubble, due ...
We present a review of wave packet dynamics in different systems and stress their relation to information on the ultrafast structural changes. We show how dynamical information is obtained from ultrafast optical pump-probe studies on structural changes in ...
A wide variety of physical and chemical processes at the molecular level, as charge or energy transfer, solvation, electronic as well as vibrational relaxation, is at the origin of the biological functionality of proteins. The work reported in this thesis ...
For understanding the behavior of a gas close to a channel wall it is important to model the gas-wall interactions as detailed as possible. When using molecular dynamics simulations these interactions can be modeled explicitly, but the computations are tim ...