Ghost imaging

Ghost imaging (also called "coincidence imaging", "two-photon imaging" or "correlated-photon imaging") is a technique that produces an of an object by combining information from two light detectors: a conventional, multi-pixel detector that doesn't view the object, and a single-pixel (bucket) detector that does view the object. Two techniques have been demonstrated. A quantum method uses a source of pairs of entangled photons, each pair shared between the two detectors, while a classical method uses a pair of correlated coherent beams without exploiting entanglement. Both approaches may be understood within the framework of a single theory. History The first demonstration of ghost imaging, performed by T. B. Pittman, Y. H. Shih, D. V. Strekalov, and A. V. Sergienko in 1995, was based on quantum correlations between entangled photon pairs. One of the photons of the pair strikes the object and then the bucket detector while the other follows a different path to a (multi-p

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Attosecond transient absorption spooktroscopy: a ghost imaging approach to ultrafast absorption spectroscopy

Andre Al Haddad, Christoph Bostedt, Jonas Knurr, Siqi Li

The recent demonstration of isolated attosecond pulses from an X-ray free-electron laser (XFEL) opens the possibility for probing ultrafast electron dynamics at X-ray wavelengths. An established experimental method for probing ultrafast dynamics is X-ray transient absorption spectroscopy, where the X-ray absorption spectrum is measured by scanning the central photon energy and recording the resultant photoproducts. The spectral bandwidth inherent to attosecond pulses is wide compared to the resonant features typically probed, which generally precludes the application of this technique in the attosecond regime. In this paper we propose and demonstrate a new technique to conduct transient absorption spectroscopy with broad bandwidth attosecond pulses with the aid of ghost imaging, recovering sub-bandwidth resolution in photoproduct-based absorption measurements.

ROYAL SOC CHEMISTRY2020

Optically reconfigurable quasi-phase-matching in silicon nitride microresonators

Camille Sophie Brès, Jianqi Hu, Edgars Nitiss, Anton Stroganov

Quasi-phase-matching has long been a widely used approach in nonlinear photonics, enabling efficient parametric frequency conversions such as second-harmonic generation. However, in silicon photonics the task remains challenging, as materials best suited for photonic integration lack second-order susceptibility (χ(2)), and means for achieving momentum conservation are limited. Here we present optically reconfigurable quasi-phase-matching in large-radius silicon nitride microresonators, resulting in up to 12.5-mW on-chip second-harmonic generated power and a conversion efficiency of 47.6% W−1. Most importantly, we show that such all-optical poling can occur unconstrained from intermodal phase-matching, leading to broadly tunable second-harmonic generation. We confirm the phenomenon by two-photon imaging of the inscribed χ(2) grating structures within the microresonators as well as by in situ tracking of both the pump and second-harmonic mode resonances during all-optical poling. These results unambiguously establish that the photogalvanic effect, responsible for all-optical poling, can overcome phase mismatch constraints, even in resonant systems.

2022

Harmonic Nanoparticles for Regenerative Research

Luigi Bonacina, Jérôme Extermann, Jean-Pierre Wolf

In this visualized experiment, protocol details are provided for in vitro labeling of human embryonic stem cells (hESC) with second harmonic generation nanoparticles (HNPs). The latter are a new family of probes recently introduced for labeling biological samples for multi-photon imaging. HNPs are capable of doubling the frequency of excitation light by the nonlinear optical process of second harmonic generation with no restriction on the excitation wavelength. Multi-photon based methodologies for hESC differentiation into cardiac clusters (maintained as long term air-liquid cultures) are presented in detail. In particular, evidence on how to maximize the intense second harmonic (SH) emission of isolated HNPs during 3D monitoring of beating cardiac tissue in 3D is shown. The analysis of the resulting images to retrieve 3D displacement patterns is also detailed.

Journal Of Visualized Experiments2014

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