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We report on the generation of broadband, high-energy femtosecond pulses centered at 1.28 mu m by stimulated Raman scattering in a pressurized hydrogen cell. Stimulated Raman scattering is performed by two chirped and delayed pulses originating from a mult ...
Controlled mixtures of novel Mg-based metal-organic frameworks (MOFs) were prepared, with H+ or K+ as counterions. A linear relation was found between synthesis pH and K/H ratio in the resultant mixture, establishing the tunability of the synthesis. Upon p ...
When large volumes of fluids are removed from or injected into underground formations for, e.g., hydrocarbon and water production, CO_2 storage, gas storage, and geothermal energy exploitation, monitoring of surface deformations coupled to numerical modeli ...
The interplay of secondary hydrogen bonds of 2- and 3-ethynylpyridine or ethynylbenzene with trimethylphosphate in tetrachloroethene was elucidated using FT-Raman spectroscopy and MP2/6-311 + G(d,p) calculations. The direct participation of C C moiety in t ...
Organic semiconductors have been proven to be suitable for efficient photovoltaic generation during the last decade but have been scarcely assessed as photoelectrochemical devices. In this work we present the fabrication and characterization of a new effic ...
CO2 sequestration in deep geological formations is considered as a promising technology to reduce the impact of CO2 on the greenhouse effect. Practically, large-volume of CO2 could be injected into a system that consists of a highly porous host reservoir c ...
Geomechanical stability issues may arise due to induced thermal stresses because CO2 will generally reach the storage formation at a temperature lower than that of the reservoir. Cold injection will form a cold region around the injection well, which will ...
We apply first-principles approaches with Hubbard U corrections for calculation of small molecule binding energetics to open-shell transition metal atoms in metal-organic frameworks (MOFs). Using density functional theory with van derWaals dispersion-corre ...
Folk wisdom usually takes the number of participants as an often necessary and sufficient condition for identifying a crowd. This assumption has diffused among academics interested in crowdsourcing and collective intelligence as well. Yet, consider 50 peop ...
A combined experimental-numerical approach was used to study transient phenomena occurring in a photoelectrochemical cell using a membrane-separated porous TiO2-based photoanode and a dark Pt-based cathode. The effects of three parameters (pH in the anodic ...
