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Optically Transparent FTO-Free Cathode for Dye-Sensitized Solar Cells

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Two new metal-free organic sensitizers, L156 and L224, were designed, synthesized, and characterized for application in dye-sensitized solar cells (DSCs). The structures of the dyes contain a triphenylamine (TPA) segment and 4-(benzo[c][1,2,5]thiadiazol-4- ...

WILEY-V C H VERLAG GMBH2019

Influence of Ionic Liquid Electrolytes on the Photovoltaic Performance of Dye-Sensitized Solar Cells

Shaik Mohammed Zakeeruddin, Jean-David Décoppet

New binary ionic liquid electrolytes based on 1-methyl-1-butylpyrrolidinium bis(trifluromethylsulfonyl)imide, 1-butylpyridinium bis(trifluromethylsulfonyl)imide, 1-methyl-3-ethylimidazolium bis(trifluromethylsulfonyl)imide, 1-methyl-3-ethylimidazolium tetr ...

Wiley-V C H Verlag Gmbh2017

Electrochemical Properties of Cu(II/I)-Based Redox Mediators for Dye-Sensitized Solar Cells

Shaik Mohammed Zakeeruddin, Ulf Anders Hagfeldt, Ladislav Kavan, Yasemin Saygili, Marina Freitag

Three Cu(II/I)-phenanthroline and Cu(II/I)-bipyridine redox mediators are studied on various electrodes and in variety of electrolyte solutions using cyclic voltammetry and impedance spectroscopy on symmetrical dummy cells. Graphene-based catalysts provide ...

2017

A small electron donor in cobalt complex electrolyte significantly improves efficiency in dye-sensitized solar cells

Lei Zhang, Ulf Anders Hagfeldt, Yan Hao, Yasemin Saygili

Photoelectrochemical approach to solar energy conversion demands a kinetic optimization of various light-induced electron transfer processes. Of great importance are the redox mediator systems accomplishing the electron transfer processes at the semiconduc ...

Nature Publishing Group2016

Donor design and modification strategies of metal-free sensitizers for highly-efficient n-type dye-sensitized solar cells

Xiaoyu Zhang

Dye-sensitized solar cells (DSSCs) cannot be developed without the research on sensitizers. As the key of light harvesting and electron generation, thousands of sensitizers have been designed for the application in DSSC devices. Among them, organic sensiti ...

Higher Education Press2016

Phthalocyanines (Pcs) are used as sensitizers in dye-sensitized solar cells (DSSCs) because of their stability and intense absorption in the red and near-IR regions. Impressive progress has been made in photovoltaic efficiencies by introduction of bulky pe ...

Wiley-V C H Verlag Gmbh2016

A new photoelectrochromic device (PECD) is presented in this work proposing the combination of a WO3-based electrochromic device (ECD) and a polymer-based dye-sensitized solar cell (DSSC). In the newly designed architecture, a photocurable polymeric membra ...

Wiley-Blackwell2016

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An ullazine unit was employed as a donor moiety in a donor-pi-acceptor (D-p-A) motif, employing the porphyrin macrocycle as a pi-system. Synthesis of this ullazine-porphyrin dyad containing sensitizer (SM63) was achieved and an investigation of the electro ...

2016

Copper Phenanthroline as a Fast and High-Performance Redox Mediator for Dye-Sensitized Solar Cells

Michael Graetzel, Fabrizio Giordano, Ulf Anders Hagfeldt, Yan Hao, Marina Freitag

The most commonly used redox mediators in dye-sensitized solar cells (DSCs), iodide/triiodide and cobalt trisbipyridine (Co(bpy)(3)), were successfully replaced by bis (2,9-dimethy1-1,10-phenanthroline) copp er (I/H) (Cu(dmp)(2)). The use ...

American Chemical Society2016

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Interfaces of dye-sensitized TiO2 nanoparticles with electrolytes or hole conductors have been widely applied in photoelectrochemical cells. However, the fundamental understanding of their properties and function is still poor. Herein, we demonstrate that ...

American Chemical Society2016