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Comprehensive control of voltage loss enables 11.7% efficient solid-state dye-sensitized solar cells

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Photoelectrochemical Cell Engineering for Solar Energy Conversion

Dan Zhang

Solar energy is the most abundant energy source, harnessing solar energy holds the solution to the challenge of increasing global energy demand and reducing our dependence on fossil fuels. Photovoltaics which directly convert solar energy into electricity ...

EPFL2023

The teachings herein relate to hole transport compounds containing cyclobutyl moieties that can be made into organic hole conductors and hole transport materials. Furthermore, optoelectronic and photoelectrochemical devices, in particular photovoltaic devi ...

2023

All-inorganic halide perovskites for air-processed "n-i-p" monolithic perovskite/organic hybrid tandem solar cells exceeding 23% efficiency

Mohammad Khaja Nazeeruddin

All-perovskite tandem solar cells recently surpassed 26% power conversion efficiency using a Sn(ii)-based halide perovskite rear subcell, which introduces several issues related to the chemical instability and the effectiveness of common, inexpensive inter ...

Cambridge2023

Photoinduced charge separation into free carriers and subsequent charge transfer are key processes that govern the efficiencies of third generation solar cell technologies based on donor-acceptor heterojunctions. As these processes typically occur on picos ...

2022

Molecular Engineering of Fluorene-Based Hole-Transporting Materials for Efficient Perovskite Solar Cells

Mohammad Khaja Nazeeruddin, Hiroyuki Kanda, Albertus Adrian Sutanto, Nadja Isabelle Desiree Klipfel

New Spiro-OMeTAD analogues and the simpler "half" structures with the terminated methoxyphenyl and/or carbazolyl chromophores are successfully synthesized under Hartwig-Buchwald amination conditions using commercially available starting materials. New fluo ...

WILEY-V C H VERLAG GMBH2022

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Photosensitizers yielding superior photocurrents are crucial for copper-electrolyte-based highly efficient dye-sensitized solar cells (DSCs). Herein, two molecularly tailored organic sensitizers are presented, coded ZS4 and ZS5, through judiciously employi ...

WILEY-V C H VERLAG GMBH2022

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Inorganic perovskite solar cells (PSCs) have witnessed extraordinary advances owing to their prominent stability against thermal aging. However, they suffer from a phase transition from black phase to yellow phase under ambient conditions and serious energ ...

WILEY-V C H VERLAG GMBH2022

Cation optimization for burn-in loss-free perovskite solar devices

Mohammad Khaja Nazeeruddin, Sanghyun Paek, Cristina Roldán Carmona, Marius Franckevicius, Olga Syzgantseva

Hybrid lead halide perovskites will potentially lead the future energy scenario if highly efficient cells have long-term stability. Here we combine state-of-the art mixed-cation formulations containing formamidinium (FA) and methylammonium (MA), with optim ...

2021

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One of the most prominent hole-transporting material (HTM) for hybrid perovskite solar cells has been 2,2″,7,7″-tetrakis[N,N-di(4-methoxyphenyl)amino]-9,9′-spirobifluorene (spiro-OMeTAD), which is commonly doped with metal bis(trifluoromethylsulfonyl)imide ...

2021

Chenodeoxycholic acid (CDCA) is the most used antiaggregation additive in dye-sensitized solar cells since its introduction to the field in 1993. However, effective suppression of dye aggregation comes at the cost of reduced dye loading, a lower open-circu ...

WILEY-V C H VERLAG GMBH2020