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Segregation of Nickel/Iron Bimetallic Particles from Lanthanum Doped Strontium Titanates to Improve Sulfur Stability of Solid Oxide Fuel Cell Anodes

Related publications (51)

Spinel Protective Coatings for Solid Oxide Cell (SOC) Interconnects (ICs)

AbstractThe degradation of metal interconnects (ICs) in Solid Oxide Cells (SOCs) primarily results from chromium (Cr) oxide scale growth on stainless-steel substrates, causing ohmic loss and air-side electrode poisoning by Cr. This thesis addresses these c ...

EPFL2024

Cu/Metal Oxide Hybrid Nanocrystals as Electrocatalysts for the CO2 Reduction Reaction

Seyedehbehnaz Varandili

The electrochemical CO2 reduction reaction (CO2RR) is envisioned to play a significant role in achieving carbon neutrality while contributing to storing renewable energies. Cu-based materials are among the most promising electrocatalysts. However, 16 diffe ...

EPFL2021

Performance Analysis of Ammonia in Solid Oxide Fuel Cells

Jan Van Herle, Suhas Nuggehalli Sampathkumar, Peter Hugh Middleton, Steve Joris

Ammonia (NH3) has 17.8 wt% hydrogen and is easily liquified at 25°C and 8 bar pressure. Ammonia is carbon-free and can be produced sustainably at large scale and low cost. Solid oxide fuel cells generate electricity with efficiencies greater than 60% and c ...

ECS2021

Increased nickel exsolution from LaFe0.8Ni0.2O3 perovskite-derived CO2 methanation catalysts through strontium doping

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Perovskite-derived Ni catalysts offer the remarkable benefit of redox stability that allows their regeneration after deactivation through poisoning or Ni particle growth. Here, the catalytic activity of LaFe0.8Ni0.2O3 towards CO2 methanation was improved b ...

ELSEVIER2020

Oxygen evolution reaction catalyzed by first-row transition metal oxides: stability and mechanism

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Water splitting offers the opportunity for storing solar energy and, thus, producing carbon-neutral and renewable solar fuels. The process, known as artificial photosynthesis, is limited by the electrocatalytic conversion of water into molecular oxygen. El ...

EPFL2020

Molecular Engineering of Electrode Surfaces for Electrocatalysis

Patrick Eduard Alexa

Electrocatalysts play an important part on the route towards environmental friendly energy sources. They support modern technologies like fuel cells to move further away from the utilization of fossil fuels and the resulting CO2 emission into our atmospher ...

EPFL2020

Efficient Hydrogen Oxidation Catalyzed by Strain-Engineered Nickel Nanoparticles

Xile Hu, Pascal Alexander Schouwink, Weiyan Ni, Teng Wang

The hydroxide-exchange membrane fuel cell (HEMFC) is a promising energy conversion device. However, the development of HEMFC is hampered by the lack of platinum-group-metal-free (PGM-free) electrocatalysts for the hydrogen oxidation reaction (HOR). Now, a ...

WILEY-V C H VERLAG GMBH2020

Segregation of Nickel/Iron Bimetallic Particles from Lanthanum Doped Strontium Titanates to Improve Sulfur Stability of Solid Oxide Fuel Cell Anodes

Davide Ferri, Oliver Kröcher, Andre Heel

Perovskite derived Ni catalysts offer the remarkable benefit of regeneration after catalyst poisoning or Ni particle growth through the reversible segregation of Ni from the perovskite-type oxide host. Although this property allows for repeated catalyst re ...

MDPI2019

Sulfur Poisoning Recovery on a Solid Oxide Fuel Cell Anode Material through Reversible Segregation of Nickel

Jan Van Herle, Davide Ferri, Oliver Kröcher, Hossein Madi, Andre Heel

The perovskite-type mixed oxide La0.3Sr0.55Ti0.95Ni0.05O3-delta (LSTN) is demonstrated to exhibit the remarkable property of structural regeneration, where Ni can be reversibly exsoluted from the host perovskite lattice resulting in a regenerable Ni cataly ...

AMER CHEMICAL SOC2019

Stability of metallo-porphyrin networks under oxygen reduction and evolution conditions in alkaline media

Klaus Kern, Jan Gui-Hyon Dreiser, Markus Etzkorn, Claudius Morchutt, Sebastian Stepanow, Benjamin Wurster

Transition metal atoms stabilised by organic ligands or as oxides exhibit promising catalytic activity for the electrocatalytic reduction and evolution of oxygen. Built-up from earth-abundant elements, they offer affordable alternatives to precious-metal b ...

2019

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