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Unconventional Spin Relaxation Involving Localized Vibrational Modes in Ho Single-Atom Magnets

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Spin excitations and quantum criticality in the quasi-one-dimensional Ising-like ferromagnet CoCl2⋅2D2O in a transverse field

Henrik Moodysson Rønnow, Ursula Bengaard Hansen

We present experimental evidence for a quantum phase transition in the easy-axis S=3/2 anisotropic quasi-one-dimensional ferromagnet CoCl2⋅2D2O in a transverse field. Elastic neutron scattering shows that the magnetic order parameter vanishes at a transver ...

2017

Direct enhancement of nitrogen-15 targets at high-field by fast ADAPT-SABRE

Gabriele Stevanato

Signal Amplification by Reversible Exchange (SABRE) is an attractive nuclear spin hyperpolarization technique capable of huge sensitivity enhancement in nuclear magnetic resonance (NMR) detection. The resonance condition of SABRE hyperpolarization depends ...

2017

Controlling the Spin of Co Atoms on Pt(111) by Hydrogen Adsorption

Harald Brune, Christian Wäckerlin, Pietro Gambardella, Fabio Donati, Markus Etzkorn, Anne Lehnert, Quentin Dubout, Laurent Claude

We investigate the effect of H adsorption on the magnetic properties of individual Co atoms on Pt(111) with scanning tunneling microscopy. For pristine Co atoms, we detect no inelastic features in the tunnel spectra. Conversely, CoH and CoH2 show a number ...

Amer Physical Soc2015

Rotation-induced recovery and bleaching in magnetic resonance

Geoffrey Bodenhausen, Diego Carnevale, Angel Joaquin Perez Linde, Srinivas Chinthalapalli

Thurber and Tycko recently described a 'bleaching effect' that occurs in magnetic resonance when solid samples that are doped with paramagnetic agents are subjected to rotation by magic angle spinning (MAS) in a static magnetic field with a rotation period ...

Royal Society of Chemistry2015

We report that the electron spin-relaxation time T1 in a GaAs quantum dot with a spin-1/2 ground state has a 180° periodicity in the orientation of the in-plane magnetic field. This periodicity has been predicted for circular dots as being due to the inter ...

2014

Spin processes and charge dynamics in organic light emitting diodes

Francesco Comandè

In this thesis work we explore spin dependent processes and charge dynamics in α-NPD/Alq₃ based LEDs. Studies on polymer light emitting diodes based on PFO, which are fabricated by us, are also reported. Our objective is to shed light on the fundamental me ...

EPFL2014

Modifying the properties of 4f single-ion magnets by peripheral ligand functionalisation

Jan Gui-Hyon Dreiser

We study the ligand-field splittings and magnetic properties of three Er-III single-ion magnets which differ in the peripheral ligand sphere but exhibit similar first coordination spheres by inelastic neutron scattering (INS) and SQUID magnetometry. The IN ...

Royal Soc Chemistry2014

In this thesis, we present development of the first magnetic model of the main Proton Synchrotron magnets. The operation of the machine and conducting research on increasing its performance require a significant amount of the magnetic field data for the op ...

EPFL2013

Intriguing aspects of lanthanide luminescence

Jean-Claude Bünzli, Svetlana Eliseeva

The enthralling properties of lanthanide luminescence have propelled luminescent probes, tags and materials based on these elements to the forefront of science and technology. In this minireview, attention is focused on the latest innovations and on less-k ...

Royal Soc Chemistry2013

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The high intrinsic spin and long spin relaxation time of manganese-12-acetate (Mn-12) makes it an archetypical single molecular magnet. While these characteristics have been measured on bulk samples, questions remain whether the magnetic properties replica ...

2012