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Surface, Interface, and Bulk Electronic and Chemical Properties of Complete Perovskite Solar Cells: Tapered Cross-Section Photoelectron Spectroscopy, a Novel Solution

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The properties of efficient solar cells fabricated with triple-cation perovskite placed between a mesoporous titania layer and a spiro-OMeTAD layer are studied by using devices either prepared under water-free drybox conditions or fabricated under ambient ...

AMER CHEMICAL SOC2020

All-inorganic perovskite films hold promise for improving stability of perovskite solar cells. However, the desirable narrow-bandgap inorganic perovskites (such as CsPbI3 and CsPbI2Br) are suffering from the thermodynamic phase instability, as the photoact ...

EPFL2020

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The emerging 2D perovskites exhibit superior stability and similar optoelectronic attributes compared to the 3D analogues, but their strong exciton-binding energy and inferior interlayer charge-transport reduce dramatically the device performance. Herein, ...

2020

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Since reaching 20% efficiency, research in perovskite photovoltaics has shifted from a race for efficiency to a race for stability. For efficiency, the standard test conditions set the rules for the race. However, the term 'stability' is used very broadly ...

NATURE PUBLISHING GROUP2019

A chain is as strong as its weakest link - Stability study of MAPbI(3) under light and temperature

Michael Graetzel, Ulf Anders Hagfeldt, Michael Saliba, Pankaj Kumar Yadav, Amita Ummadisingu, Silver Hamill Turren Cruz, Philippe Jürgen Holzhey

The stability of perovskite solar cells is a key issue for industrial development. One reason for this is the volatile organic methylammonium (MA) cation, which is prone to degas under elevated temperatures from the perovskite. At the same time, small amou ...

2019

I-2 vapor-induced degradation of formamidinium lead iodide based perovskite solar cells under heat-light soaking conditions

Christophe Ballif, Quentin Thomas Jeangros, Adriana Paracchino, Sylvain Nicolay, Jérémie Werner, Fan Fu, Peter Joseph Fiala, Léo Duchêne

Over the last years, the operational stability of perovskite solar cells has been significantly improved by compositional engineering, interface modification, and improved encapsulation techniques. However, irreversible degradation is still ubiquitously ob ...

2019

The strategy of mixing cations and halides in hybrid organic lead halide perovskites has recently been shown to be very successful in achieving high efficiency with long-term perovskite solar cell stability. In this study, the effect of photoexcitation on ...

WILEY-V C H VERLAG GMBH2019

Perovskite solar cells (PSCs) have attracted a substantial interest owing to a very fast achievement of efficiencies >20 % within only several years of development. However, for any solar cell to become technologically viable, two additional milestones hav ...

EPFL2018

Compositional Characterization of Organo-Lead tri-Halide Perovskite Solar Cells

Paul Gratia

Perovskite photovoltaics is one of the fastest growing research fields in materials science. Apart from photovoltaics, a wide range of energy-related research fields have gained substan-tial new momentum owing to the fantastic optoelectronic properties of ...

EPFL2018

Water-Repellent Low-Dimensional Fluorous Perovskite as Interfacial Coating for 20% Efficient Solar Cells

Mohammad Khaja Nazeeruddin, Yi Zhang, Andreas Stephan Lesch, Iwan Zimmermann, Giulia Grancini, Kyung Taek Cho

Hybrid perovskite solar cells have been capturing an enormous research interest in the energy sector due to their extraordinary performances and ease of fabrication. However, low device lifetime, mainly due to material and device degradation upon water exp ...

2018