Vibrationally inelastic scattering of HCl from Ag(111)
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Magnetic skyrmions are whirl-like spin configurations with particle-like properties protected by non-trivial topology. Due to their unique spin structures and dynamical properties, they have attracted tremendous interests over the past decade, from fundame ...
In this thesis, I describe the design and implementation of the first state-to-state surface scattering experiments for methane from clean single crystalline surfaces in ultrahigh vacuum. The experiments use infrared laser pumping to prepare the incident C ...
State-to-state molecule/surface scattering experiments prepare the incident molecules in a specific quantum state and measure the quantum state distribution of the scattered molecules. The comparison of state resolved experiments with theory can serve as s ...
This thesis presents a quantum-state-resolved molecular beam study of the non-reactive scattering of methane (CH4) from a Ni(111) surface. It is one of the first experimental investigations in which the internal quantum state distribution of a polyatomic m ...
The phenomenology of resonant scattering has been known since the earliest experiments upon scattering of atomic beams from surfaces and is a means of obtaining experimental information about the fundamentals of weak adsorption systems in the van der Waals ...
In this thesis, I present an experimental molecular beam surface scattering study of dynamical processes involved when HCl molecules are scattered from Au(111) and Ag(111) surfaces. I investigated vibrational excitation, translational inelasticity and diss ...
The fate of vibrational energy in the collision of methane (CH4) in its antisymmetric C-H stretch vibration (ν3) with a Ni(111) surface has been studied in a state-to-state scattering experiment. Laser excitation in the incident molecular beam prepared the ...
We describe a novel UHV state-to-state molecule/surface scattering apparatus with quan- tum state preparation of the incident molecular beam and angle-resolved quantum state detection of the scattered molecules. State resolved detection is accomplished usi ...
Spin-orbit changing transitions for bond-axis oriented collisions of NO(X) with Ar have been investigated with full quantum state selection via a crossed molecular beam experiment at collision energies of 532 cm(-1) and 651 cm(-1). NO(X) molecules were sel ...
Quantum state-resolved scattering experiments for methane molecules colliding with a catalytically active nickel surface are compared to scattering from a nickel surface passivated by a single layer of graphene. The vibrational state distribution of the sc ...