Photodissociation studies of CH3I and CF3I in fluid 4Helium nanodroplets
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We show how a relativistic effective field theory for the superfluid phase of 4 He can replace the standard methods used to compute the production rates of low-momentum excitations due to the interaction with an external probe. This is done by studying the ...
We employ an effective field theory to study the detectability of sub-GeV dark matter through its interaction with the gapless excitations of superfluid 4He. In a quantum field theory language, the possible interactions between the dark matter and the supe ...
I present a molecular beam study of methane dissociation on differ-ent surface sites of several platinum single crystal surfaces (Pt(111), Pt(211), Pt(210), Pt(110)-(2x1)). The experiments were performed in a molecular beam/surface-science apparatus that c ...
This thesis presents a quantum-state-resolved molecular beam study of the non-reactive scattering of methane (CH4) from a Ni(111) surface. It is one of the first experimental investigations in which the internal quantum state distribution of a polyatomic m ...
The properties of nanometric-sized helium bubbles in silicon have been investigated using both spatially resolved electron-energy-loss spectroscopy combined with a recently developed method, and molecular-dynamics simulations. The experiments allowed for a ...
The possibility for helium-induced electronic transitions in a photo-excited atom is investigated using Ba+ excited to the 6p 2P state as a prototypical example. A diabatization scheme has been designed to obtain the necessary potential energy surfaces and ...
In this work we seek to examine the nature of collisional energy transfer between HCl and Au(111) for nonreactive scattering events that sample geometries near the transition state for dissociative adsorption by varying both the vibrational and translation ...
Path integral methods provide a rigorous and systematically convergent framework to include the quantum mechanical nature of atomic nuclei in the evaluation of the equilibrium properties of molecules, liquids, or solids at finite temperature. Such nuclear ...
We consider a general approach for the process of Lagrangian and Hamiltonian reduction by symmetries in chiral gauge models. This approach is used to show the complete integrability of several one dimensional texture equations arising in liquid Helium phas ...
Non-local effects have been traditionally identified as one of the most limiting factors of the performance of Brillouin optical time-domain analyzers. These phenomena, directly linked with the energy gained/lost by the pump pulse, limit the probe power an ...