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The ultrafast dynamics are reported of bubble formation following excitation of the A 2S+ 3ss(v = 0) Rydberg state of NO trapped in Ar matrixes. The study is carried out by a fs pump-probe technique. The detected signal is the depletion of Rydberg fluorescence induced by Rydberg-Rydberg transitions. Possibly the bubble is formed on a timescale of a few ps. [on SciFinder (R)]
Basil Duval, Christian Gabriel Theiler, Artur Perek, Kevin Henricus Annemarie Verhaegh, Mirko Wensing
Frédéric Mila, Samuel Louis Nyckees
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