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One-step hydroxylation of benzene to phenol by N2O has been performed over structured catalytic beds made of ZSM-5 coatings on stainless steel grids. The catalysts demonstrated high activity with a selectivity toward phenol formation of 98%. A detailed kinetic study was carried out with a variation in reactant concentrations, benzene/N2O ratio, and residence time. The results obtained suggest a surface reaction between benzene and nitrous oxide adsorbed on two different active sites.
Jeremy Luterbacher, Jher Hau Yeap, Bartosz Rozmyslowicz, Ahmed Mohamed Ibrahim Elkhaiary
Andreas Osterwalder, Bruno Credidio
Karen Scrivener, Paul Bowen, Maya Nicole Harris, Grace Simpson