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The total synthesis of pentacyclic monoterpene indole alkaloids is the focus of this thesis.
Total syntheses of (±)-alstilobanine C, (±)-undulifoline and (±)-alstilobanine B, three natural products from the Ulean family of alkaloids, were accomplished. The ...
Utilization of edge devices has exploded in the last decade, with such use cases as wearable devices, autonomous driving, and smart homes. As their ubiquity grows, so do expectations of their capabilities. Simultaneously, their formfactor and use cases lim ...
The Materials Genome Approach (MGA) aims to accelerate development of new materials by incorporating computational and data-driven approaches to reduce the cost of identification of optimal structures for a given application. Here, we use the MGA to guide ...
Product vacua with boundary states (PVBS) are cousins of the Heisenberg XXZ spin model and feature [Formula: see text] particle species on [Formula: see text]. The PVBS models were originally introduced as toy models for the classification of ground state ...
The present invention concerns a method of generating setpoints for actuators (13) of a real-time control system. The method comprises a first controller (9): a) receiving a first set of measurements from sensors (3), the measurements being individually la ...
The structure of uleine type alkaloids is characterized by the presence of a bridged tetracyclic hexahydro-1H-1,5-methanoazocino[4,3-b]indole ring system 1. Various strategies have been developed to access this polycyclic structural motif. We report herein ...
Motivated by the remarkable properties of SrCu2(BO3)(2) in a magnetic field, we use perturbative continuous unitary transformations to determine the magnetization plateaux of the Shastry-Sutherland model, unveiling an unexpected sequence of plateaux progre ...
Given two video sequences, a composite video sequence can be generated which includes visual elements from each of the given sequences, suitably synchronized and represented in a chosen focal plane. For example, given two video sequences with each showing ...
Given two video sequences, a composite video sequence can be generated which includes visual elements from each of the given sequences, suitably synchronized and represented in a chosen focal plane. For example, given two video sequences with each showing ...
Motivated by the presence of Ising transitions that take place entirely in the singlet sector of frustrated spin-1/2 ladders and spin-1 chains, we study two types of effective dimer models on ladders, a quantum dimer model and a quantum loop model. Buildin ...