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Carbon dioxide may constitute a source of chemicals and fuels if efficient and renewable processes are developed that directly utilize it as feedstock. Two of its reduction products are formic acid and methanol, which have also been proposed as liquid orga ...
Securing our energy future while minimizing the associated environmental impacts is a challenging endeavor and the fundamental aspect of sustainable development. The choice of energy resource and the reduction of greenhouse gas emissions, primarily carbon ...
Oxidation kinetics of iodide and HOI/OI- by permanganate were studied in the pH range of 5.0-10.0. Iodide oxidation and iodate formation were faster at lower pH. The apparent second-order rate constants (k(obs)) for iodide oxidation by permanganate decreas ...
The invention relates to a method for producing methanol from hydrogen and carbon dioxide gas in homogeneously catalyzed reactions, composed of the carbon dioxide hydrogenation reaction to formic acid and the formic acid disproportionation reaction into me ...
Horseradish peroxidase (HRP) is one of the most relevant peroxidase enzymes, used extensively in immunochemistry and biocatalysis applications. Unlike the closely related catalase enzymes, it exhibits a low activity to disproportionate hydrogen peroxide (H ...
Multimetallic cooperative binding of heteroallenes provides an attractive route to their activation, but the reduction of CS2 at heterobimetallic sites, associating an electron-rich metal with a main group Lewis acid has not been explored. Here we show tha ...
The lactone motif is ubiquitous in natural products and pharmaceuticals. The Tishchenko disproportionation of two aldehydes, a carbonyl hydroacylation, is an efficient and atom-economic access to lactones. However, these reaction types are limited to the t ...
Olivine-type LiCoPO4 (LCP) is a high energy density lithium ion battery cathode material due to the high voltage of the Co2+/Co3+ redox reaction. However, it displays a significantly poorer electrochemical performance than its more widely investigated isos ...
Bromate formation from the reaction between chlorine and bromide in homogeneous solution is a slow process. The present study investigated metal oxides enhanced bromate formation during chlorination of bromide-containing waters. Selected metal oxides enhan ...
Nucleic acid synthesis is spatially organized in many organisms. In bacteria, however, the spatial distribution of transcription remains obscure, owing largely to the diffraction limit of conventional light microscopy (200-300 nm). Here, we use photoactiva ...