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Hydrogen sieving from intrinsic defects of benzene-derived single-layer graphene

Kumar Varoon Agrawal, Mostapha Dakhchoune, Shiqi Huang, Jing Zhao, Mina Moradi, Majharul Haque Khan

Single-layer graphene films, crystallized by chemical vapor deposition, host a low density of vacancy defects that are attractive for the size-sieving of molecules. The size and the density of such defects are a function of the growth temperature and the c ...

2019

Electrochemical Behavior of Carbon Electrodes for In Situ Redox Studies in a Transmission Electron Microscope

Vasiliki Tileli, Robin Pierre Alain Girod, Nikolaos Nianias

Electrochemical liquid cell transmission electron microscopy (TEM) is a unique technique for probing nanocatalyst behavior during operation for a range of different electrocatalytic processes, including hydrogen evolution reaction (HER), oxygen evolution r ...

CAMBRIDGE UNIV PRESS2019

Enhanced Sensing of Interleukin 8 by Stripping Voltammetry: Carbon Nanotubes versus Fullerene

Sandro Carrara, Tugba Kilic, Sarah Tonello

The ability to detect protein biomarkers at a subnanomolar level represents a pervasive challenge in order to bring a significant improvement in early diagnosis or progression of pato-physiological processes. To this aim, Screen Printed Electrochemical Sen ...

SPRINGER-VERLAG SINGAPORE PTE LTD2018

Photosensitized Hydrogen Evolution on a Floating Electrocatalyst Coupled to Electrochemical Recycling

Hubert Girault, Astrid Johana Olaya Avendano, Jonnathan Cesar Hidalgo Acosta, Terumasa Omatsu

Photoexcited protonated tetrathiafulvalene (HTTF+) was found to act as a photosensitizer, injecting electrons into Pt microparticles (floating electrocatalysts) to produce H2 and TTF•+ in acidic acetonitrile. In addition, TTF•+ was electrochemically reduce ...

2018

Influence of Ablation on Vacuum-Ultraviolet Radiation in a Plasma Wind Tunnel Flow

Pénélope Leyland

Plasma wind tunnel experiments have been performed simulating a Hayabusa reentry trajectory point at 78.8km altitude with a velocity of 11.7km/s corresponding to a local mass-specific enthalpy of 68.4MJ/kg and a stagnation pressure of 2.44kPa. Ablation-rad ...

American Institute of Aeronautics and Astronautics2017

Multimaterial Nanoporous Membranes Shaped through High Aspect-Ratio Sacrificial Silicon Nanostructures

Philippe Renaud, Arnaud Bertsch, Niccolo Piacentini, Stefano Silvio Giovanni Varricchio

We present an innovative fabrication method for solid-state nanoporous membranes based on the casting of sacrificial silicon nanostructures. The process allows the individual definition of geometry and placement of each nanopore through e-beam lithography ...

Amer Chemical Soc2017

On the Limits of Precision Glass Molding for Diffractive Optical Elements

Karin Prater

Diffractive optical elements (DOEs) consist of surface reliefs with dimensions in the micrometer range and nanometer precision. Two technologies dominate: Elements replicated in plastic and directly microfabricated elements in fused silica. Plastic DOEs ar ...

EPFL2017

Columnar self-assembly of N,N ',N ''-trihexylbenzene-1,3,5-tricarboxamides investigated by means of NMR spectroscopy and computational methods in solution and the solid state

Diego Carnevale, Mathieu Baudin

The columnar self-assembly resulting from units of N, N', N"-trihexylbenzene-1,3,5-tricarboxamide is investigated in solution and the solid state by means of NMR spectroscopy. A parallel computational study utilizing both semiempirical and DFT methods allo ...

Royal Soc Chemistry2017

Precision glass molding of high-resolution diffractive optical elements

Hans Peter Herzig, Toralf Scharf, Karin Prater

The demand of high resolution diffractive optical elements (DOE) is growing. Smaller critical dimensions allow higher deflection angles and can fulfill more demanding requirements, which can only be met by using electron-beam lithography. Replication techn ...

Spie-Int Soc Optical Engineering2016

Order/Disorder Dynamics in a Dodecanethiol-Capped Gold Nanoparticles Supracrystal by Small-Angle Ultrafast Electron Diffraction

Francesco Stellacci, Fabrizio Carbone, Giulia Fulvia Mancini, Tatiana Latychevskaia, Francesco Pennacchio, Javier Reguera Gomez

The design and the characterization of functionalized gold nanoparticles supracrystals require atomically resolved information on both the metallic core and the external organic ligand shell. At present, there is no known approach to characterize simultane ...

American Chemical Society2016

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