Isolant topologique | EPFL Graph Search

Un isolant topologique est un matériau ayant une structure de bande de type isolant mais qui possède des états de surface métalliques. Ces matériaux sont donc isolants "en volume" et conducteurs en surface. Historique En 2007, cet état de matière a été réalisé pour la première fois en 2D dans un puits quantique de (Hg,Cd)Te . Le BiSb (antimoniure de bismuth) est le premier isolant topologique 3D à être réalisé. La spectroscopie de photoélectrons résolue en angle a été l'outil principal qui a servi à confirmer l'existence de l'état isolant topologique en 3D. À la suite de ces deux découvertes, une troisième génération d'isolants topologiques a vu le jour. La manipulation dangereuse de certains éléments comme le mercure et l'antimoine encouragea plusieurs groupes à rechercher des matériaux plus sûrs et plus faciles à produire comme le Bi2Se3 ou bien le Bi2Te3. Peu après la découverte du BiSb, les états de surface du Bi2Se3 ont été observés. À présent, quelques matériaux ca

Charge transport properties of spin-orbit coupled materials in different correlation regimes

Soudabeh Sheikholharam Mashhadi

From recent advances in solid state physics, a novel material classification scheme has evolved which is based on the concept of topology and provides an understanding of different phenomena ranging from quantum transport to unusual flavors of superconductivity. Spin-orbit coupling is a major term in defining the topology of materials, and its interplay with electron electron correlations yields novel, intriguing phenomena. In the weak to intermediate correlation regime, spin-orbital entanglement leads to the emergence of topological insulators, which constitute Dirac materials with 2D spin-polarized helical edge or surface states and an insulating bulk. In the specific case of topological insulators, theory predicts that their unique band structure leads to a high thermoelectric performance, which is of practical relevance for energy conversion applications.In the strong correlation regime, the spin-orbit coupling removes the orbital degeneracy, thereby enhancing quantum fluctuations of the spin-orbit entangled states. This in turn can lead to the emergence of novel phases such as quantum spin liquids and unconventional superconductivity. The Kitaev quantum spin liquid (QSL) is a topological state of matter that exhibits fractionalized excitations in the form of Majorana fermions. The main aim of this thesis was to study these novel states of matter in the form of two different materials that fall in the weak and strong correlation regime, respectively. On this basis, it should furthermore be explored whether benefit can be taken of their properties by combining them with other quantum materials into heterostructures.In the first part of this thesis, nanoplatelets of bismuth chalcogenide-based 3D topological insulators were grown by chemical vapor deposition, and characterized by magnetotransport experiments. Having established charge transport characteristics of the single components, in the aim to exploit their high thermoelectric efficiency, the lateral heteroctructures of them are fabricated. Their investigation by scanning photocurrent microscopy revealed strong photocurrent generation at the p-n junction. The obtained results demonstrate that such type of hybrid heterostructure is a promising route to enhance the thermoelectric performance in nanostructured devices. In the second part of this thesis, the Kitaev spin liquid candidate, RuCl3 was studied. Raman spectroscopy on exfoliated RuCl3 revealed a broad magnetic continuumat low energies which according to its particular deviation from bosonic character is assigned to the fractionalized excitations. Furthermore, in complementary charge transport experiments, it was found that themagnetic fluctuations and structural changes in thismaterial are highly entangled, and influence the emergence of the fractionalized excitations. Finally, it was investigated whether the magnetic insulator character of ®-RuCl3 can be exploited to alter the graphene band structure through a proximity effect in vertical graphene/ RuCl3 heterostructures. Measurements of their low-temperature, nonlocal resistance confirmed the possibility to induce pure spin currents in this manner. At the same time, the charge transport through the graphene served as a probe of the magnetic ordering in RuCl3, although the complex magnetic behavior in this material necessitates more studies.

EPFL2018

Charge transport in proximitized graphene within van der Waals heterostructures

Katharina Polyudov

Since their discovery, graphene and other 2D materials have become a subject of intense research in condensed matter physics. Especially the vast possibilities of combining those materials into heterostructures are promising for the discovery of novel physical phenomena. The heterostructures accessible through state-of-the-art techniques have suitably clean interfaces between the layers. Graphene has gained a lot of attention due to its remarkable mechanical stability and extremely high electron mobility. However, the zero bandgap of graphene is a major bottleneck for implementing this 2D material into most electronic applications. The ability to tune the properties of graphene by proximity effects has shifted the focus of graphene research towards the combination of graphene with other van der Waals materials. The main objective of the present thesis was to explore for two different types of graphene-based van der Waals heterostructure whether fingerprints of electronic proximity effects can be traced in their low temperature magnetotransport properties. The first part of the thesis deals with heterostructures of graphene and Bi2Te2Se (BTS). The strong spin-orbit coupling of BTS makes it a three-dimensional topological insulator with topological surface states which are protected by time-reversal symmetry. At the same time, BTS is promising to exert a pronounced spin-orbit proximity effect on graphene, and thereby to open a band gap and/or introduce a spin texture in the latter. The graphene/BTS heterostructures were fabricated by the direct growth of BTS on graphene to ensure a clean interface between both materials and correspondingly a good electronic coupling between them. Analysis of the weak localization effect observed in the magnetoconductivity revealed the presence of enhanced SOC in the proximitized graphene. The second part of the thesis focuses on heterostructures wherein graphene is combined with a-RuCl3 which has recently gained a lot of attention as a potential quantum spin liquid system. Previous studies on graphene/a-RuCl3 heterostructures found an unusual temperature evolution of the quantum oscillation amplitude, whose origin remained unclear. The magnetotransport data collected in this thesis point toward two possible origins for this behavior, namely spin fluctuations associated with the magnetic transition into an antiferromagnetic phase at the Néel temperature of approximately 7 K, and the hybridization-induced formation of heavy (flat) bands, both of which are likely to depend on the a-RuCl3 layer thickness. In addition, heterostructures comprising an a-RuCl3 monolayer were found to display a unusual gate dependence of the quantum oscillations, further corroborating the importance of the a-RuCl3 thickness.

EPFL2020

Theories of topologically-induced phenomena in skyrmion-hosting magnetoelectric insulators

Oleksandr Kriuchkov

There once was a harsh competition between different computer memory technologies, and now we cheer triumph for the Random Access-Memory (RAM) devices, -- cheap, fast, tiny, stable. The competing Magnetic Bubble Memory had faded away as magnetic bubbles are undesirably large and pretty much not robust, manifesting both low data density and high operational costs. However, what we do possess now are nanosize objects of topological nature, magnetic skyrmions, which are protected from continuous field variations and take very little energy cost to be moved. Thus, skyrmions are considered as promising information carriers for future memory devices and ultradense data storage, while skyrmion phases in bulk materials are interesting from fundamental point of view in exploring topological states of matter. In this thesis, I develop and advance several effective theoretical approaches, diverse both in their methods and use, which were of appeal for several skyrmionic experiments in our lab (LQM/EPFL). We were and are primarily interested in the open issues in the applied field of skyrmionics, which may be taken under the umbrella of creation, stabilization and control of magnetic skyrmions under electric fields, mechanical strains, thermal gradients, etc. For the goals achieved and yet to be achieved, the magnetoelectric insulator Cu2OSeO3, which uniquely responses to all the above mentioned fields, is a highly advantageous candidate. Magnetoelectric here means that the spins of a magnetic material are coupled to external electric fields, while insulating properties are very advantageous to preserve both the state and the very existence of skyrmions by eliminating the Joule heating. The novel results in this thesis are calculations for both individual and arrayed skyrmions under electric fields, mechanical strains and uniform pressures, and thermal gradients. Furthermore, several fundamental questions were addressed by developing an extended formalism for calculation skyrmion-pocket phase diagrams, studying the topologically-governed crossover between skyrmions and magnetic bubbles, and discussing the possible role of merons (half-skyrmions) in skyrmion phase formation. The result with the most immediate appeal is probably the theoretical and experimental study of skyrmion lattices in electric fields, with a direct demonstration of writing and erasing of the full skyrmion phase under electric fields of few Volts per micrometer, as compatible with modern microelectronic devices.

EPFL2017