Publications associées à Fission products (by element)

Atomic level insight into irradiation effects in nuclear fuel materials

Microstructural evolution during in-pile irradiation, radiation damage effects and fission products behavior in UO2 nuclear fuel are key issues in understanding and for the modeling of the performance as well as safety characteristics of nuclear fuels in t ...

EPFL2024

Gamma-ray Spectroscopy in Low-Power Nuclear Research Reactors

Andreas Pautz, Vincent Pierre Lamirand, Oskari Ville Pakari

Gamma-ray spectroscopy is an effective technique for radioactive material characterization, routine inventory verification, nuclear safeguards, health physics, and source search scenarios. Gamma-ray spectrometers typically cannot be operated in the immedia ...

MDPI2024

A concept for the extraction of the most refractory elements at CERN-ISOLDE as carbonyl complex ions

João Pedro Fernandes Pinto Ramos

We introduce a novel thick-target concept tailored to the extraction of refractory 4d and 5d transition metal radionuclides of molybdenum, technetium, ruthenium and tungsten for radioactive ion beam production. Despite the more than 60-year old history of ...

2022

Interface Tracking Investigation of the Sliding Bubbles Effects on Heat Transfer in the Laminar Regime

Konstantin Mikityuk, Lubomír Bures

Helium gases are utilized to remove fission products from the molten salt fast reactor (MSFR) core during operation. Helium gases and other volatile fission products may be introduced into the intermediate heat exchanger channels. The effect of these gases ...

2022

Towards the Validation of Noise Experiments in the CROCUS Reactor Using the TRIPOLI-4 Monte Carlo Code in Analog Mode

Andreas Pautz, Vincent Pierre Lamirand, Oskari Ville Pakari

Intrinsic neutron noise experiments offer a non-invasive manner to measure the prompt decay constant or reactivity of fissile systems. Using the fluctuations in the density of fission chains, one can infer the kinetics parameters via correlation analysis s ...

2021

High-Efficiency Deep-Red Light-Emitting Electrochemical Cell Based on a Trinuclear Ruthenium(II)-Silver(I) Complex

Mohammad Khaja Nazeeruddin

Turn-on time is a key factor for lighting devices to be of practical application. To decrease the turn-on time value of a deep-red light-emitting electrochemical cells (DR-LECs), two novel approaches based on molecularly engineered ruthenium phenanthroimid ...

AMER CHEMICAL SOC2021

Data assimilation of post-irradiation examination data for fission yields from GEF

Andreas Pautz, Daniel Jerôme Siefman, Mathieu Hursin, Dimitri Rochman

Nuclear data, especially fission yields, create uncertainties in the predicted concentrations of fission products in spent fuel which can exceed engineering target accuracies. Herein, we present a new framework that extends data assimilation methods to bur ...

EDP SCIENCES S A2020

Data assimilation of post irradiation examination experiments to adjust fission yields

Andreas Pautz, Daniel Jerôme Siefman, Mathieu Hursin

Nuclear data, especially fission yields, create uncertainties in the predicted concentrations of fission products in spent fuel. Herein, we present a new framework that extends data assimilation methods to burnup simulations by using data from post-irradia ...

E D P SCIENCES2020

Artificial Neural Networks as Surrogate Models for Uncertainty Quantification and Data Assimilation in 2-D/3-D Fuel Performance Studies

Andreas Pautz, Mathieu Hursin, Carlo Fiorina, Alessandro Scolaro, Daniel Jerôme Siefman

This paper preliminarily investigates the use of data-driven surrogates for fuel performance codes. The objective is to develop fast-running models that can be used in the frame of uncertainty quantification and data assimilation studies. In particular, da ...

2020

Nuclear data uncertainties for Swiss BWR spent nuclear fuel characteristics

Mathieu Hursin, Hakim Ferroukhi, Dimitri Rochman, Abdelhamid Dokhane, Alexander Vasiliev

The effect of nuclear data (fission yields, cross sections and emitted spectra) is quantified for spent nuclear fuel assemblies from a realistic boiling water reactor operated over 25 cycles. Nominal calculations are performed with the CASMO5, SIMULATE-3 a ...

2020