Concept

Potentiel quantique

Publications associées (38)

Revealing higher-order light and matter energy exchanges using quantum trajectories in ultrastrong coupling

The dynamics of open quantum systems is often modeled using master equations, which describe the expected outcome of an experiment (i.e., the average over many realizations of the same dynamics). Quantum trajectories, instead, model the outcome of ideal si ...

AMER PHYSICAL SOC2022

Engineering and characterizing nonclassical states of light in quantum optical networks

Kilian Robert Seibold

The exploration of open quantum many-body systems -systems of microscopic size exhibiting quantum coherence and interacting with their surrounding- has emerged as a key research area over the last years. The recent advances in controlling and preserving qu ...

EPFL2022

Simulating the ghost: quantum dynamics of the solvated electron

Michele Ceriotti, Jinggang Lan, Venkat Kapil, Piero Gasparotto

The nature of the bulk hydrated electron has been a challenge for both experiment and theory due to its short lifetime and high reactivity, and the need for a high-level of electronic structure theory to achieve predictive accuracy. The lack of a classical ...

2021

Superexchange mechanism and quantum many body excitations in the archetypal di-Cu oxo-bridge

Edward Baxter Linscott, Cédric Weber

The hemocyanin protein binds and transports molecular oxygen via two copper atoms at its core. The singlet state of the Cu2O2 core is thought to be stabilised by a superexchange pathway, but detailed in situ computational analysis is complicated by the mul ...

NATURE PUBLISHING GROUP2020

On-the-Fly ab initio Semiclassical Evaluation of Electronic Coherences in Polyatomic Molecules Reveals a Simple Mechanism of Decoherence

Jiri Vanicek, Tomislav Begusic, Nikolay Golubev

Irradiation of a molecular system by an intense laser field can trigger dynamics of both electronic and nuclear subsystems. The lighter electrons usually move on much faster, attosecond timescale but the slow nuclear rearrangement damps ultrafast electroni ...

2020

Sign-Changing Solutions for a Class of Zero Mass Nonlocal Schrodinger Equations

We consider the following class of fractional Schrodinger equations: (-Delta)(alpha)u + V(x)u = K(x)f(u) in R-N, where alpha is an element of (0, 1), N > 2 alpha, (-Delta)(alpha) is the fractional Laplacian, V and K are positive continuous functions which ...

2019

The electronic interface for quantum processors

Edoardo Charbon, Fabio Sebastiano

Quantum computers can potentially provide an unprecedented speed-up with respect to traditional computers. However, a significant increase in the number of quantum bits (qubits) and their performance is required to demonstrate such quantum supremacy. While ...

ELSEVIER SCIENCE BV2019

Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators

Tobias Kippenberg, Clément Christian Javerzac-Galy, Ryan Daniel Schilling, Sina Khorasani, Nicolas Piro Mastracchio, Anshuman Kumar

We present quantum yield measurements of single layer WSe2 (1L-WSe2) integrated with high-Q (Q > 106) optical microdisk cavities, using an efficient (η > 90%) near-field coupling scheme based on a tapered optical fiber. Coupling of the excitonic emission i ...

2018

Intrinsic structure of pentapeptide Leu-enkephalin: geometry optimization and validation by comparison of VSCF-PT2 calculations with cold ion spectroscopy

Vladimir Kopysov, Oleg Boyarkine, Aleksandr Pereverzev, Robert Benny Gerber

The intrinsic structure of an opioid peptide [Ala2, Leu5]-leucine enkephalin (ALE) has been investigated using first-principles based vibrational self-consistent field (VSCF) theory and cold ion spectroscopy. IR-UV double resonance spectroscopy revealed th ...

2018

Geometric Integrators for Nonadiabatic Molecular Quantum Dynamics Induced by the Interaction with the Electromagnetic Field

Aurélien Kevin Fabrice Patoz

Understanding the elementary steps involved in a chemical reaction forms the cornerstone of physical chemistry research. One way to deepen this understanding is by studying chemical and physical processes using linear and nonlinear spectroscopic techniques ...

EPFL2017

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