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4 f occupancy and magnetism of rare-earth atoms adsorbed on metal substrates

Publications associées (52)

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We examine the diffusion of methane in the metal organic frameworks M-2(dobdc) (M = Mg, Ni, Zn; dobdc(4-) = 2,5-diwddo-1,4-benzenedicarboxylate) as a function of methane loading through a combination of nuclear magnetic resonance and molecular dynamics sim ...

2019

Magnetic exchange parameters and anisotropy of the quasi-two-dimensional antiferromagnet NiPS3

Diane Virginie Marie Lançon

Neutron inelastic scattering has been used to measure the magnetic excitations in powdered NiPS3, a quasitwo-dimensional antiferromagnet with spin S = 1 on a honeycomb lattice. The spectra show clear, dispersive magnons with a similar to 7 meV gap at the B ...

AMER PHYSICAL SOC2018

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Activated carbon fibers (ACFs) with surface modified by a diethylene triamine (DETA) are synthesized for the abatement of formaldehyde in gas phase at low concentration. Adsorbents with several DETA loadings were tested and characterized. The amount of DET ...

2018

Magnetic properties of surface-adsorbed single rare earth atoms, molecules, and atomic scale clusters

Aparajita Singha

This thesis presents combined experimental and theoretical investigations of nanoscale, surface-supported magnets based on rare earths (RE) to understand and control the magnetic properties down to the scale of single atoms. We present the effects of adato ...

EPFL2017

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We demonstrate that electrospray deposition enables the fabrication of highly periodic self-assembled arrays of Fe4H single molecule magnets on graphene/Ir(111). The energetic positions of molecular states are probed by means of scanning tunneling spectros ...

American Chemical Society2017

Reading and writing single-atom magnets

Donat Fabian Natterer

The single-atom bit represents the ultimate limit of the classical approach to high-density magnetic storage media. So far, the smallest individually addressable bistable magnetic bits have consisted of 3-12 atoms(1-3). Long magnetic relaxation times have ...

Nature Publishing Group2017

The removal of sulfur compounds in biomass gasification processes is crucial to protect downstream equipment. While conventional sorbent materials can retain H2S, many fail to capture heterocyclic sulfur compounds such as thiophene (C4H4S). This work explo ...

Elsevier Sci Ltd2017

Exploring the relevance of gas-phase structures to biology: cold ion spectroscopy of the decapeptide neurokinin A

Aleksandr Pereverzev

Linking the intrinsic tertiary structures of biomolecules to their native geometries is a central prerequisite for making gas-phase studies directly relevant to biology. The isolation of molecules in the gas phase eliminates hydrophilic interactions with s ...

Royal Society of Chemistry2017

Magnetic Hysteresis in Er Trimers on Cu(111)

Harald Brune, Stefano Rusponi, Marina Pivetta, Christian Wäckerlin, Jan Gui-Hyon Dreiser, Fabio Donati, Aparajita Singha, Romana Baltic

We report magnetic hysteresis in Er clusters on. Cu(111) starting from the size-of three atoms. combining Xray magnetic circular dichroism, scanning tunneling microscopy, and mean-field nucleation theory, we determine the size dependent magnetic properties ...

American Chemical Society2016

Superlattice of Single Atom Magnets on Graphene

Harald Brune, Stefano Rusponi, Marina Pivetta, Christian Wäckerlin, Jan Gui-Hyon Dreiser, Fabio Donati, Aparajita Singha, Romana Baltic

Regular arrays of single atoms with stable magnetization represent the ultimate limit of ultrahigh density storage media. Here we report a self-assembled superlattice of individual and noninteracting Dy atoms on graphene grown on Ir(111), with magnetic hys ...

American Chemical Society2016