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Tzu-Hsien Shen

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Related publications (9)

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Insights into Electrocatalyst Transformations Studied in Real Time with Electrochemical Liquid-Phase Transmission Electron Microscopy

Vasiliki Tileli, Tzu-Hsien Shen, Robin Pierre Alain Girod

The value of operando and in situ characterization methodologies for understanding electrochemical systems under operation can be inferred from the upsurge of studies that have reported mechanistic insights into electrocatalytic processes based on such mea ...

Washington2023

Electron probing of oxygen-evolving oxide catalysts

Tzu-Hsien Shen

Water splitting is one of the cleanest ways to store energy. The production of hydrogen and oxygen gases can be utilized in fuel cells to generate electricity, power, and heat. In the water splitting process, the oxygen evolution reaction (OER), taking pla ...

EPFL2022

Switchable wetting of oxygen-evolving oxide catalysts

Vasiliki Tileli, Tzu-Hsien Shen

The surface wettability of catalysts is typically controlled via surface treatments that promote catalytic performance. Here we report on potential-regulated hydrophobicity/hydrophilicity at cobalt-based oxide interfaces with an alkaline solution. The swit ...

NATURE PORTFOLIO2021

Multi-channel nanowire devices for efficient power conversion

Elison de Nazareth Matioli, Vasiliki Tileli, Tzu-Hsien Shen

Nanowire-based devices can potentially be of use in a variety of electronic applications, from ultrascaled digital circuits to 5G communication networks. However, the devices are typically restricted to low-power applications due to the relatively low elec ...

NATURE RESEARCH2021

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Electrochemical liquid-phase transmission electron microscopy (TEM) is showing excellent promise in fundamental studies of energy-related processes including lithium-ion battery (LIB) cycling. A key requirement to accurately interpret the measurements and ...

2020

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Among the perovskites used to catalyze the oxygen evolution reaction (OER), Ba0.5Sr0.5Co0.8Fe0.2O3-delta (BSCF) exhibits excellent activity which is thought to be related to dynamic reconstruction at the flexible perovskite surface due to accommodation of ...

AMER CHEMICAL SOC2020

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Size, morphology, and surface sites of electrocatalysts have a major impact on their performance. Understanding how, when, and why these parameters change under operating conditions is of importance for designing stable, active, and selective catalysts. He ...

WILEY-V C H VERLAG GMBH2020

Charge/discharge cycling of Li1+x(Ni0.6Co0.2Mn0.2)1−xO2 primary particles performed in a liquid microcell for transmission electron microscopy studies

Vasiliki Tileli, Tzu-Hsien Shen, Robin Pierre Alain Girod, Jing Hou

Ni-rich layered oxides are promising positive electrodes for fulfillment of government and industry targets for lithium-ion-battery-operated electric mobility purposes. Apart from ongoing research focusing on their design and material production, advanced ...

2020

Impact of Intermittent Operation on Lifetime and Performance of a PEM Water Electrolyzer

Vasiliki Tileli, Tzu-Hsien Shen

The aim of this study is to provide a better understanding of performance degrading mechanisms occurring when a proton exchange membrane water electrolyzer (PEM-WE) is coupled with renewable energies, where times of operation and idle periods alternate. An ...

ELECTROCHEMICAL SOC INC2019