Global Identification of Kinetic Parameters via the Extent-based Incremental Approach
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The reaction of aldehydes, amines and TMSCN in the presence of 2-iodoxybenzoic acid (IBX) and tetrabutylammonium bromide (TBAB) afforded alpha -iminonitriles, e.g. 4-MeOC6H4C(C==N):NCH2CH2Ph, in good to excellent yields under mild conditions. The presence ...
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The synthesis of the alkoxide [OC(tBu)(CF3)2]− by the reaction of tBuM-reagents (M = Li; MgX) with hexafluoroacetone was attempted. This alkoxide was anticipated to be a good building block for novel weakly coordinating anions. However, in all attempted sy ...
Kinetic hard-modelling of multivariate spectroscopic data [1, 2] is a well-established method for the determination of reaction mechanisms and associated rate constants. Kinetic hard-modelling relies on a hard model defined by kinetic rate laws and require ...
Abstract--- In this paper we describe a new class of representations for real-valued parameters called Center of Mass Encoding (CoME). CoME is based on variable length strings, it is self-adaptive, and it permits the choice of the degree of redundancy of t ...
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An efficient synthesis of functionalized 3-alkyl-3-cyanomethyl-2-oxindole by a palladium-catalyzed domino Heck-cyanation reaction has been developed. Reaction of ortho-iodoanilide with potassium ferro(II)cyanide in the presence of palladium acetate and sod ...
Investigations of spectrum adjustment by unfolding techniques for different locations of critical and driven subcritical MUSE4 configurations are presented. The current analysis is based on the recent accomplishment of specific foil activation measurements ...